Observation of the anomalous Nernst effect in altermagnetic candidate Mn5Si3

Fuente: arXiv
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Autori principali: Badura, Antonin, Campos, Warlley H., Bharadwaj, Venkata K., Kounta, Ismaïla, Michez, Lisa, Petit, Matthieu, Rial, Javier, Leiviskä, Miina, Baltz, Vincent, Krizek, Filip, Kriegner, Dominik, Zemen, Jan, Telkamp, Sjoerd, Sailler, Sebastian, Lammel, Michaela, Ubiergo, Rodrigo Jaeschke, Hellenes, Anna Birk, González-Hernández, Rafael, Sinova, Jairo, Jungwirth, Tomáš, Goennenwein, Sebastian T. B., Šmejkal, Libor, Reichlova, Helena
Natura: Preprint
Pubblicazione: 2024
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author Badura, Antonin
Campos, Warlley H.
Bharadwaj, Venkata K.
Kounta, Ismaïla
Michez, Lisa
Petit, Matthieu
Rial, Javier
Leiviskä, Miina
Baltz, Vincent
Krizek, Filip
Kriegner, Dominik
Zemen, Jan
Telkamp, Sjoerd
Sailler, Sebastian
Lammel, Michaela
Ubiergo, Rodrigo Jaeschke
Hellenes, Anna Birk
González-Hernández, Rafael
Sinova, Jairo
Jungwirth, Tomáš
Goennenwein, Sebastian T. B.
Šmejkal, Libor
Reichlova, Helena
author_facet Badura, Antonin
Campos, Warlley H.
Bharadwaj, Venkata K.
Kounta, Ismaïla
Michez, Lisa
Petit, Matthieu
Rial, Javier
Leiviskä, Miina
Baltz, Vincent
Krizek, Filip
Kriegner, Dominik
Zemen, Jan
Telkamp, Sjoerd
Sailler, Sebastian
Lammel, Michaela
Ubiergo, Rodrigo Jaeschke
Hellenes, Anna Birk
González-Hernández, Rafael
Sinova, Jairo
Jungwirth, Tomáš
Goennenwein, Sebastian T. B.
Šmejkal, Libor
Reichlova, Helena
contents The anomalous Nernst effect generates transverse voltage to the applied thermal gradient in magnetically ordered systems. The effect was previously considered excluded in compensated magnetic materials with collinear ordering. However, in the recently identified class of compensated magnetic materials, dubbed altermagnets, time-reversal symmetry breaking in the electronic band structure makes the presence of the anomalous Nernst effect possible despite the collinear spin arrangement. In this work, we investigate epitaxial Mn5Si3 thin films known to be an altermagnetic candidate. We show that the material manifests a sizable anomalous Nernst coefficient despite the small net magnetization of the films. The measured magnitudes of the anomalous Nernst coefficient reach a scale of microVolts per Kelvin. We support our magneto-thermoelectric measurements by density-functional theory calculations of the material's spin-split electronic structure, which allows for the finite Berry curvature in the reciprocal space. Furthermore, we present our calculations of the intrinsic Berry-curvature Nernst conductivity, which agree with our experimental observations.
format Preprint
id arxiv_https___arxiv_org_abs_2403_12929
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Observation of the anomalous Nernst effect in altermagnetic candidate Mn5Si3
Badura, Antonin
Campos, Warlley H.
Bharadwaj, Venkata K.
Kounta, Ismaïla
Michez, Lisa
Petit, Matthieu
Rial, Javier
Leiviskä, Miina
Baltz, Vincent
Krizek, Filip
Kriegner, Dominik
Zemen, Jan
Telkamp, Sjoerd
Sailler, Sebastian
Lammel, Michaela
Ubiergo, Rodrigo Jaeschke
Hellenes, Anna Birk
González-Hernández, Rafael
Sinova, Jairo
Jungwirth, Tomáš
Goennenwein, Sebastian T. B.
Šmejkal, Libor
Reichlova, Helena
Materials Science
Mesoscale and Nanoscale Physics
The anomalous Nernst effect generates transverse voltage to the applied thermal gradient in magnetically ordered systems. The effect was previously considered excluded in compensated magnetic materials with collinear ordering. However, in the recently identified class of compensated magnetic materials, dubbed altermagnets, time-reversal symmetry breaking in the electronic band structure makes the presence of the anomalous Nernst effect possible despite the collinear spin arrangement. In this work, we investigate epitaxial Mn5Si3 thin films known to be an altermagnetic candidate. We show that the material manifests a sizable anomalous Nernst coefficient despite the small net magnetization of the films. The measured magnitudes of the anomalous Nernst coefficient reach a scale of microVolts per Kelvin. We support our magneto-thermoelectric measurements by density-functional theory calculations of the material's spin-split electronic structure, which allows for the finite Berry curvature in the reciprocal space. Furthermore, we present our calculations of the intrinsic Berry-curvature Nernst conductivity, which agree with our experimental observations.
title Observation of the anomalous Nernst effect in altermagnetic candidate Mn5Si3
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2403.12929