Toward Optimum Coupling between Free Electrons and Confined Optical Modes
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arXiv
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| Auteurs principaux: | , , , |
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| Format: | Preprint |
| Publié: |
2024
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| _version_ | 1866918145146486784 |
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| author | Di Giulio, Valerio Akerboom, Evelijn Polman, Albert de Abajo, F. Javier García |
| author_facet | Di Giulio, Valerio Akerboom, Evelijn Polman, Albert de Abajo, F. Javier García |
| contents | Free electrons are unique tools to probe and manipulate nanoscale optical fields with emerging applications in ultrafast spectromicroscopy and quantum metrology. However, advances in this field are hindered by the small probability associated with the excitation of single optical modes by individual free electrons. Here, we theoretically investigate the scaling properties of the electron-driven excitation probability for a wide variety of optical modes including plasmons in metallic nanostructures and Mie resonances in dielectric cavities, spanning a broad spectral range that extends from the ultraviolet to the infrared. The highest probabilities for the direct generation of three-dimensionally confined modes are observed at low electron and mode energies in small structures, with order-unity ($\sim100$\%) coupling demanding the use of $<100$~eV electrons interacting with $<1$~eV polaritons confined down to tens of nm. Electronic transitions in artificial atoms also emerge as practical systems to realize strong coupling to few-eV free electrons. In contrast, conventional dielectric cavities reach a maximum probability in the few-percent range. In addition, we show that waveguide modes can be generated with higher-than-unity efficiency by phase-matched interaction with grazing electrons, suggesting an efficient method to create multiple excitations of a localized optical mode by an individual electron through funneling the so-generated propagating photons into a confining cavity -- an alternative approach to direct electron-cavity interaction. Our work provides a roadmap to optimize electron-photon coupling with potential applications in electron spectromicroscopy as well as nonlinear and quantum optics at the nanoscale. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2403_15823 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | Toward Optimum Coupling between Free Electrons and Confined Optical Modes Di Giulio, Valerio Akerboom, Evelijn Polman, Albert de Abajo, F. Javier García Optics Mesoscale and Nanoscale Physics Free electrons are unique tools to probe and manipulate nanoscale optical fields with emerging applications in ultrafast spectromicroscopy and quantum metrology. However, advances in this field are hindered by the small probability associated with the excitation of single optical modes by individual free electrons. Here, we theoretically investigate the scaling properties of the electron-driven excitation probability for a wide variety of optical modes including plasmons in metallic nanostructures and Mie resonances in dielectric cavities, spanning a broad spectral range that extends from the ultraviolet to the infrared. The highest probabilities for the direct generation of three-dimensionally confined modes are observed at low electron and mode energies in small structures, with order-unity ($\sim100$\%) coupling demanding the use of $<100$~eV electrons interacting with $<1$~eV polaritons confined down to tens of nm. Electronic transitions in artificial atoms also emerge as practical systems to realize strong coupling to few-eV free electrons. In contrast, conventional dielectric cavities reach a maximum probability in the few-percent range. In addition, we show that waveguide modes can be generated with higher-than-unity efficiency by phase-matched interaction with grazing electrons, suggesting an efficient method to create multiple excitations of a localized optical mode by an individual electron through funneling the so-generated propagating photons into a confining cavity -- an alternative approach to direct electron-cavity interaction. Our work provides a roadmap to optimize electron-photon coupling with potential applications in electron spectromicroscopy as well as nonlinear and quantum optics at the nanoscale. |
| title | Toward Optimum Coupling between Free Electrons and Confined Optical Modes |
| topic | Optics Mesoscale and Nanoscale Physics |
| url | https://arxiv.org/abs/2403.15823 |