Detection of spin pumping free of rectification and thermal artefacts in molecular-based ferromagnetic insulator V[TCNE]x~2

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Main Authors: Wang, Zichen, Kurfman, Seth, Ursel, Sarah, Johnston-Halperin, E., Sirringhaus, Henning
Format: Preprint
Published: 2024
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_version_ 1866913289299034112
author Wang, Zichen
Kurfman, Seth
Ursel, Sarah
Johnston-Halperin, E.
Sirringhaus, Henning
author_facet Wang, Zichen
Kurfman, Seth
Ursel, Sarah
Johnston-Halperin, E.
Sirringhaus, Henning
contents The molecular-based ferrimagnetic insulator V(TCNE)x has gained recent interest for efficient spin-wave excitation due to its low Gilbert damping ratio a=4E-5, and narrow ferromagnetic resonance linewidth f=1Oe. Here we report a clean spin pumping signal detected on V(TCNE)x/metal bilayer structures, free from spin rectification or thermal artifacts. On-chip coupling of microwave power is achieved via a coplanar waveguide to measure the in-plane angle-dependence of the inverse spin-Hall effect under ferromagnetic resonance conditions with respect to a constant external magnetic field. A signature of pure spin current from V(TCNE)x is observed in both platinum and permalloy metal layers, demonstrating the utility of V(TCNE)x for magnon spintronics studies in molecule/solid-state heterostructures.
format Preprint
id arxiv_https___arxiv_org_abs_2403_16429
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Detection of spin pumping free of rectification and thermal artefacts in molecular-based ferromagnetic insulator V[TCNE]x~2
Wang, Zichen
Kurfman, Seth
Ursel, Sarah
Johnston-Halperin, E.
Sirringhaus, Henning
Materials Science
The molecular-based ferrimagnetic insulator V(TCNE)x has gained recent interest for efficient spin-wave excitation due to its low Gilbert damping ratio a=4E-5, and narrow ferromagnetic resonance linewidth f=1Oe. Here we report a clean spin pumping signal detected on V(TCNE)x/metal bilayer structures, free from spin rectification or thermal artifacts. On-chip coupling of microwave power is achieved via a coplanar waveguide to measure the in-plane angle-dependence of the inverse spin-Hall effect under ferromagnetic resonance conditions with respect to a constant external magnetic field. A signature of pure spin current from V(TCNE)x is observed in both platinum and permalloy metal layers, demonstrating the utility of V(TCNE)x for magnon spintronics studies in molecule/solid-state heterostructures.
title Detection of spin pumping free of rectification and thermal artefacts in molecular-based ferromagnetic insulator V[TCNE]x~2
topic Materials Science
url https://arxiv.org/abs/2403.16429