Non-coplanar spin structure in a metallic thin film of triangular lattice antiferromagnet CrSe

Fuente: arXiv
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Auteurs principaux: Tajima, Yusuke, Shiogai, Junichi, Ueda, Kohei, Suzaki, Hirotake, Takaki, Kensuke, Seki, Takeshi, Kudo, Kazutaka, Matsuno, Jobu
Format: Preprint
Publié: 2024
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author Tajima, Yusuke
Shiogai, Junichi
Ueda, Kohei
Suzaki, Hirotake
Takaki, Kensuke
Seki, Takeshi
Kudo, Kazutaka
Matsuno, Jobu
author_facet Tajima, Yusuke
Shiogai, Junichi
Ueda, Kohei
Suzaki, Hirotake
Takaki, Kensuke
Seki, Takeshi
Kudo, Kazutaka
Matsuno, Jobu
contents An antiferromagnetic metal with two-dimensional triangular network offers a unique playground of intriguing magneto-transport properties and functionalities stemming from interplay between conducting electrons and intricate magnetic phases. A NiAs-type CrSe is one of the candidates owing to alternate stackings of Cr and Se triangular atomic networks in its crystal structure. While fabrication of CrSe thin films is indispensable to develop functional devices, studies on its thin-film properties have been limited to date due to the lack of metallic samples. Here, we report on realization of metallic conductivities of CrSe thin films, which allows to investigate their intrinsic magneto-transport properties. The metallic sample exhibits co-occurrence of a weak ferromagnetism with perpendicular magnetic anisotropy and the antiferromagnetic behavior, indicating the presence of non-coplanar spin structures. In addition, control of polarity and tilting angle of the non-coplanar spin structure is accomplished by a sign of cooling magnetic fields. The observed non-coplanar spin structure, which can be a source of emergent magnetic field acting on the conducting electrons, highlights a high potential of the triangular lattice antiferromagnet and provide unique platform for functional thin-film devices composed of NiAs-type derivative Cr chalcogenides and pnictides.
format Preprint
id arxiv_https___arxiv_org_abs_2403_17408
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Non-coplanar spin structure in a metallic thin film of triangular lattice antiferromagnet CrSe
Tajima, Yusuke
Shiogai, Junichi
Ueda, Kohei
Suzaki, Hirotake
Takaki, Kensuke
Seki, Takeshi
Kudo, Kazutaka
Matsuno, Jobu
Materials Science
Strongly Correlated Electrons
An antiferromagnetic metal with two-dimensional triangular network offers a unique playground of intriguing magneto-transport properties and functionalities stemming from interplay between conducting electrons and intricate magnetic phases. A NiAs-type CrSe is one of the candidates owing to alternate stackings of Cr and Se triangular atomic networks in its crystal structure. While fabrication of CrSe thin films is indispensable to develop functional devices, studies on its thin-film properties have been limited to date due to the lack of metallic samples. Here, we report on realization of metallic conductivities of CrSe thin films, which allows to investigate their intrinsic magneto-transport properties. The metallic sample exhibits co-occurrence of a weak ferromagnetism with perpendicular magnetic anisotropy and the antiferromagnetic behavior, indicating the presence of non-coplanar spin structures. In addition, control of polarity and tilting angle of the non-coplanar spin structure is accomplished by a sign of cooling magnetic fields. The observed non-coplanar spin structure, which can be a source of emergent magnetic field acting on the conducting electrons, highlights a high potential of the triangular lattice antiferromagnet and provide unique platform for functional thin-film devices composed of NiAs-type derivative Cr chalcogenides and pnictides.
title Non-coplanar spin structure in a metallic thin film of triangular lattice antiferromagnet CrSe
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2403.17408