Determination of the dynamic Young's modulus of quantum materials in piezoactuator-driven uniaxial pressure cells using a low-frequency a.c. method

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Main Authors: O'Neil, Caitlin I., Hu, Zhenhai, Kikugawa, Naoki, Sokolov, Dmitry A., Mackenzie, Andrew P., Noad, Hilary M. L., Gati, Elena
Format: Preprint
Published: 2024
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author O'Neil, Caitlin I.
Hu, Zhenhai
Kikugawa, Naoki
Sokolov, Dmitry A.
Mackenzie, Andrew P.
Noad, Hilary M. L.
Gati, Elena
author_facet O'Neil, Caitlin I.
Hu, Zhenhai
Kikugawa, Naoki
Sokolov, Dmitry A.
Mackenzie, Andrew P.
Noad, Hilary M. L.
Gati, Elena
contents We report on a new technique for measuring the dynamic Young's modulus, $E$, of quantum materials at low temperatures as a function of static tuning strain, $ε$, in piezoactuator-driven pressure cells. In addition to a static tuning of stress and strain, we apply a small-amplitude, finite-frequency a.c. (1 Hz$ \lesssim ω\lesssim $1000 Hz) uniaxial stress, $σ_{ac}$, to the sample and measure the resulting a.c. strain, $ε_{ac}$, using a capacitive sensor to obtain the associated modulus $E$. We demonstrate the performance of the new technique through proof-of-principle experiments on the unconventional superconductor Sr$_2$RuO$_4$, which is known for its rich temperature-strain phase diagram. In particular, we show that the magnitude of $E$, measured using this a.c. technique at low frequencies, exhibits a pronounced nonlinear elasticity, which is in very good agreement with previous Young's modulus measurements on Sr$_2$RuO$_4$ under [100] strain using a d.c. method (Noad et al., Science 382, 447-450 (2023)). By combining the new a.c. Young's modulus measurements with a.c. elastocaloric measurements in a single measurement, we demonstrate that these a.c. techniques are powerful in detecting small anomalies in the elastic properties of quantum materials. Finally, using the case of Sr$_2$RuO$_4$ as an example, we demonstrate how the imaginary component of the modulus can provide additional information about the nature of ordered phases.
format Preprint
id arxiv_https___arxiv_org_abs_2403_17519
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Determination of the dynamic Young's modulus of quantum materials in piezoactuator-driven uniaxial pressure cells using a low-frequency a.c. method
O'Neil, Caitlin I.
Hu, Zhenhai
Kikugawa, Naoki
Sokolov, Dmitry A.
Mackenzie, Andrew P.
Noad, Hilary M. L.
Gati, Elena
Materials Science
Strongly Correlated Electrons
Superconductivity
We report on a new technique for measuring the dynamic Young's modulus, $E$, of quantum materials at low temperatures as a function of static tuning strain, $ε$, in piezoactuator-driven pressure cells. In addition to a static tuning of stress and strain, we apply a small-amplitude, finite-frequency a.c. (1 Hz$ \lesssim ω\lesssim $1000 Hz) uniaxial stress, $σ_{ac}$, to the sample and measure the resulting a.c. strain, $ε_{ac}$, using a capacitive sensor to obtain the associated modulus $E$. We demonstrate the performance of the new technique through proof-of-principle experiments on the unconventional superconductor Sr$_2$RuO$_4$, which is known for its rich temperature-strain phase diagram. In particular, we show that the magnitude of $E$, measured using this a.c. technique at low frequencies, exhibits a pronounced nonlinear elasticity, which is in very good agreement with previous Young's modulus measurements on Sr$_2$RuO$_4$ under [100] strain using a d.c. method (Noad et al., Science 382, 447-450 (2023)). By combining the new a.c. Young's modulus measurements with a.c. elastocaloric measurements in a single measurement, we demonstrate that these a.c. techniques are powerful in detecting small anomalies in the elastic properties of quantum materials. Finally, using the case of Sr$_2$RuO$_4$ as an example, we demonstrate how the imaginary component of the modulus can provide additional information about the nature of ordered phases.
title Determination of the dynamic Young's modulus of quantum materials in piezoactuator-driven uniaxial pressure cells using a low-frequency a.c. method
topic Materials Science
Strongly Correlated Electrons
Superconductivity
url https://arxiv.org/abs/2403.17519