Theory of moiré magnetism and multi-domain spin textures in twisted Mott insulator - semimetal heterobilayers

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Main Authors: Keskiner, M. A., Ghaemi, Pouyan, Oktel, M. Ö., Erten, Onur
Format: Preprint
Published: 2024
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author Keskiner, M. A.
Ghaemi, Pouyan
Oktel, M. Ö.
Erten, Onur
author_facet Keskiner, M. A.
Ghaemi, Pouyan
Oktel, M. Ö.
Erten, Onur
contents Motivated by the recent experimental developments in van der Waals heterostructures, we investigate the emergent magnetism in Mott insulator - semimetal moiré superlattices by deriving effective spin models and exploring their phase diagram by Monte Carlo simulations. Our analysis indicates that the stacking-dependent interlayer Kondo interaction can give rise to different types of magnetic order, forming domains within the moiré unit cell. In particular, we find that the AB (AA) stacking regions tend to order (anti)ferromagnetically for an extended range of parameters. The remaining parts of the moiré unit cell form ferromagnetic chains that are coupled antiferromagnetically. We show that the decay length of the Kondo interaction can control the extent of these phases. Our results highlight the importance of stacking-dependent interlayer exchange and the rich magnetic spin textures that can be obtained in van der Waals heterostructures.
format Preprint
id arxiv_https___arxiv_org_abs_2403_18904
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Theory of moiré magnetism and multi-domain spin textures in twisted Mott insulator - semimetal heterobilayers
Keskiner, M. A.
Ghaemi, Pouyan
Oktel, M. Ö.
Erten, Onur
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Motivated by the recent experimental developments in van der Waals heterostructures, we investigate the emergent magnetism in Mott insulator - semimetal moiré superlattices by deriving effective spin models and exploring their phase diagram by Monte Carlo simulations. Our analysis indicates that the stacking-dependent interlayer Kondo interaction can give rise to different types of magnetic order, forming domains within the moiré unit cell. In particular, we find that the AB (AA) stacking regions tend to order (anti)ferromagnetically for an extended range of parameters. The remaining parts of the moiré unit cell form ferromagnetic chains that are coupled antiferromagnetically. We show that the decay length of the Kondo interaction can control the extent of these phases. Our results highlight the importance of stacking-dependent interlayer exchange and the rich magnetic spin textures that can be obtained in van der Waals heterostructures.
title Theory of moiré magnetism and multi-domain spin textures in twisted Mott insulator - semimetal heterobilayers
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2403.18904