High-temperature domain wall current in Mg-doped lithium niobate single crystals up to 400°C

Fuente: arXiv
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Auteurs principaux: Yakhnevych, Uliana, Kunzner, Marlo, Verhoff, Leonard M., Ratzenberger, Julius, Beyreuther, Elke, Rüsing, Michael, Sanna, Simone, Eng, Lukas M., Fritze, Holger
Format: Preprint
Publié: 2024
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author Yakhnevych, Uliana
Kunzner, Marlo
Verhoff, Leonard M.
Ratzenberger, Julius
Beyreuther, Elke
Rüsing, Michael
Sanna, Simone
Eng, Lukas M.
Fritze, Holger
author_facet Yakhnevych, Uliana
Kunzner, Marlo
Verhoff, Leonard M.
Ratzenberger, Julius
Beyreuther, Elke
Rüsing, Michael
Sanna, Simone
Eng, Lukas M.
Fritze, Holger
contents Conductive ferroelectric domain walls (DWs) represent a promising topical system for the development of nanoelectronic components and devices. DWs show very different properties as compared to their bulk counterparts. Of central interest here is the domain wall current (DWC) of charged DWs in 5mol\% Mg-doped lithium niobate single crystals; in contrast to former works, we extend the DWC study here to temperatures as high as 400$^\circ$C. Both the temporal stability and the thermal activation energies of 90 - 160 meV are readily deduced from current-voltage sweeps as recorded over multiple heating cycles. Our experimental work is backed up by atomistic modelling of the DWC. The latter suggests that a large band bending renders head-to-head and tail-to-tail DWs semimetallic. These detailed investigations underline the potential to extend DWC-based nanoelectronic applications even into the so-far unexplored high-temperature regime.
format Preprint
id arxiv_https___arxiv_org_abs_2404_01214
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle High-temperature domain wall current in Mg-doped lithium niobate single crystals up to 400°C
Yakhnevych, Uliana
Kunzner, Marlo
Verhoff, Leonard M.
Ratzenberger, Julius
Beyreuther, Elke
Rüsing, Michael
Sanna, Simone
Eng, Lukas M.
Fritze, Holger
Materials Science
Conductive ferroelectric domain walls (DWs) represent a promising topical system for the development of nanoelectronic components and devices. DWs show very different properties as compared to their bulk counterparts. Of central interest here is the domain wall current (DWC) of charged DWs in 5mol\% Mg-doped lithium niobate single crystals; in contrast to former works, we extend the DWC study here to temperatures as high as 400$^\circ$C. Both the temporal stability and the thermal activation energies of 90 - 160 meV are readily deduced from current-voltage sweeps as recorded over multiple heating cycles. Our experimental work is backed up by atomistic modelling of the DWC. The latter suggests that a large band bending renders head-to-head and tail-to-tail DWs semimetallic. These detailed investigations underline the potential to extend DWC-based nanoelectronic applications even into the so-far unexplored high-temperature regime.
title High-temperature domain wall current in Mg-doped lithium niobate single crystals up to 400°C
topic Materials Science
url https://arxiv.org/abs/2404.01214