The polarisation fluctuation length scale shaping the superconducting dome of SrTiO$_3$

Fuente: arXiv
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Auteurs principaux: Fauqué, Benoît, Jiang, Shan, Fennell, Tom, Roessli, Bertrand, Ivanov, Alexandre, Roux-Byl, Celine, Baptiste, Benoît, Bourges, Philippe, Behnia, Kamran, Tomioka, Yasuhide
Format: Preprint
Publié: 2024
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author Fauqué, Benoît
Jiang, Shan
Fennell, Tom
Roessli, Bertrand
Ivanov, Alexandre
Roux-Byl, Celine
Baptiste, Benoît
Bourges, Philippe
Behnia, Kamran
Tomioka, Yasuhide
author_facet Fauqué, Benoît
Jiang, Shan
Fennell, Tom
Roessli, Bertrand
Ivanov, Alexandre
Roux-Byl, Celine
Baptiste, Benoît
Bourges, Philippe
Behnia, Kamran
Tomioka, Yasuhide
contents Superconducting domes, ubiquitous across a variety of quantum materials, are often understood as a window favorite for pairing opened by the fluctuations of competing orders. Yet, a quantitative understanding of how such a window closes is missing. Here, we show that inelastic neutron scattering, by quantifying a length scale associated with polar fluctuations, $\ell_0$, addresses this issue. We find that the superconducting dome of strontium titanate definitely ends when $\ell_0$ vanishes. Moreover, the product of $\ell_0$ and the Fermi wavevector peaks close to the maximum critical temperature. Thus, this superconducting dome stems from the competition between the increase of the density of states and the unavoidable collapse of the quantum paraelectric phase, both induced by doping. The successful quantitative account of both the peak and the end of the superconducting dome implies a central role in the pairing mechanism played by the soft ferro-electric mode and its hybridisation with the acoustic branch. Such a scenario may also be at work in other quantum paraelectric materials, either bulk or interfaces.
format Preprint
id arxiv_https___arxiv_org_abs_2404_04154
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle The polarisation fluctuation length scale shaping the superconducting dome of SrTiO$_3$
Fauqué, Benoît
Jiang, Shan
Fennell, Tom
Roessli, Bertrand
Ivanov, Alexandre
Roux-Byl, Celine
Baptiste, Benoît
Bourges, Philippe
Behnia, Kamran
Tomioka, Yasuhide
Superconductivity
Strongly Correlated Electrons
Superconducting domes, ubiquitous across a variety of quantum materials, are often understood as a window favorite for pairing opened by the fluctuations of competing orders. Yet, a quantitative understanding of how such a window closes is missing. Here, we show that inelastic neutron scattering, by quantifying a length scale associated with polar fluctuations, $\ell_0$, addresses this issue. We find that the superconducting dome of strontium titanate definitely ends when $\ell_0$ vanishes. Moreover, the product of $\ell_0$ and the Fermi wavevector peaks close to the maximum critical temperature. Thus, this superconducting dome stems from the competition between the increase of the density of states and the unavoidable collapse of the quantum paraelectric phase, both induced by doping. The successful quantitative account of both the peak and the end of the superconducting dome implies a central role in the pairing mechanism played by the soft ferro-electric mode and its hybridisation with the acoustic branch. Such a scenario may also be at work in other quantum paraelectric materials, either bulk or interfaces.
title The polarisation fluctuation length scale shaping the superconducting dome of SrTiO$_3$
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2404.04154