Hidden charge density wave induced shadow bands and ultrafast dynamics of CuTe investigated using time-resolved ARPES

Fuente: arXiv
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Auteurs principaux: Zhong, Haoyuan, Bao, Changhua, Lin, Tianyun, Wang, Fei, Cai, Xuanxi, Yu, Pu, Zhou, Shuyun
Format: Preprint
Publié: 2024
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author Zhong, Haoyuan
Bao, Changhua
Lin, Tianyun
Wang, Fei
Cai, Xuanxi
Yu, Pu
Zhou, Shuyun
author_facet Zhong, Haoyuan
Bao, Changhua
Lin, Tianyun
Wang, Fei
Cai, Xuanxi
Yu, Pu
Zhou, Shuyun
contents Revealing the fine electronic structure is critical for understanding the underlying physics of low-dimensional materials. Angle-resolved photoemission spectroscopy (ARPES) is a powerful experimental technique for mapping out the experimental electronic structure. By reducing the photon energy (e.g. to 6 eV) using laser sources, a greatly improved momentum resolution can be achieved, thereby providing opportunities for ``zooming in'' the fine electronic structure and even revealing the previously unresolvable bands near the Brillouin zone center. Here, by using quasi-one-dimensional material CuTe as an example, we demonstrate the unique capability of laser-based ARPES in revealing the fine electronic structures of ``hidden'' charge density wave induced shadow bands near the Brillouin zone center, which are previously unresolvable using synchrotron sources. The observation of the shadow bands reveals the CDW phase from the aspect of band folding, and the unpredicted CDW band hybridization strongly modifies the electronic structure and Fermi surface, which suggests that such hybridization must be taken into account for studying the CDW transition. Moreover, the ultrafast non-equilibrium carrier dynamics are captured by time-resolved ARPES, revealing the relaxation dynamics through electron-phonon scattering. Our work demonstrates the advantages of laser-based ARPES in zooming in the fine electronic structures, as well as capturing the ultrafast dynamics of low-dimensional materials.
format Preprint
id arxiv_https___arxiv_org_abs_2404_05255
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Hidden charge density wave induced shadow bands and ultrafast dynamics of CuTe investigated using time-resolved ARPES
Zhong, Haoyuan
Bao, Changhua
Lin, Tianyun
Wang, Fei
Cai, Xuanxi
Yu, Pu
Zhou, Shuyun
Mesoscale and Nanoscale Physics
Revealing the fine electronic structure is critical for understanding the underlying physics of low-dimensional materials. Angle-resolved photoemission spectroscopy (ARPES) is a powerful experimental technique for mapping out the experimental electronic structure. By reducing the photon energy (e.g. to 6 eV) using laser sources, a greatly improved momentum resolution can be achieved, thereby providing opportunities for ``zooming in'' the fine electronic structure and even revealing the previously unresolvable bands near the Brillouin zone center. Here, by using quasi-one-dimensional material CuTe as an example, we demonstrate the unique capability of laser-based ARPES in revealing the fine electronic structures of ``hidden'' charge density wave induced shadow bands near the Brillouin zone center, which are previously unresolvable using synchrotron sources. The observation of the shadow bands reveals the CDW phase from the aspect of band folding, and the unpredicted CDW band hybridization strongly modifies the electronic structure and Fermi surface, which suggests that such hybridization must be taken into account for studying the CDW transition. Moreover, the ultrafast non-equilibrium carrier dynamics are captured by time-resolved ARPES, revealing the relaxation dynamics through electron-phonon scattering. Our work demonstrates the advantages of laser-based ARPES in zooming in the fine electronic structures, as well as capturing the ultrafast dynamics of low-dimensional materials.
title Hidden charge density wave induced shadow bands and ultrafast dynamics of CuTe investigated using time-resolved ARPES
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2404.05255