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Main Authors: Marcato, Tommaso, Oh, Jiwoo, Lin, Zhan-Hong, Shivarudraiah, Sunil B., Kumar, Sudhir, Zeng, Shuangshuang, Shih, Chih-Jen
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2404.05336
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author Marcato, Tommaso
Oh, Jiwoo
Lin, Zhan-Hong
Shivarudraiah, Sunil B.
Kumar, Sudhir
Zeng, Shuangshuang
Shih, Chih-Jen
author_facet Marcato, Tommaso
Oh, Jiwoo
Lin, Zhan-Hong
Shivarudraiah, Sunil B.
Kumar, Sudhir
Zeng, Shuangshuang
Shih, Chih-Jen
contents Miniaturization of light-emitting diodes (LEDs) can enable high-resolution augmented and virtual reality displays and on-chip light sources for ultra-broadband chiplet communication. However, unlike silicon scaling in electronic integrated circuits, patterning of inorganic III-V semiconductors in LEDs considerably compromises device efficiencies at submicrometer scales. Here, we present the scalable fabrication of nanoscale organic LEDs (nano-OLEDs), with the highest array density (>84,000 pixels per inch) and the smallest pixel size (~100 nm) ever reported to date. Direct nanomolecular patterning of organic semiconductors is realized by self-aligned evaporation through nanoapertures fabricated on a free-standing silicon nitride film adhering to the substrate. The average external quantum efficiencies (EQEs) extracted from a nano-OLED device of more than 4 megapixels reach up to 10%. At the subwavelength scale, individual pixels act as electroluminescent meta-atoms forming metasurfaces that directly convert electricity into modulated light. The diffractive coupling between nano-pixels enables control over the far-field emission properties, including directionality and polarization. The results presented here lay the foundation for bright surface light sources of dimension smaller than the Abbe diffraction limit, offering new technological platforms for super-resolution imaging, spectroscopy, sensing, and hybrid integrated photonics.
format Preprint
id arxiv_https___arxiv_org_abs_2404_05336
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Nanomolecular OLED Pixelization Enabling Electroluminescent Metasurfaces
Marcato, Tommaso
Oh, Jiwoo
Lin, Zhan-Hong
Shivarudraiah, Sunil B.
Kumar, Sudhir
Zeng, Shuangshuang
Shih, Chih-Jen
Optics
Materials Science
Miniaturization of light-emitting diodes (LEDs) can enable high-resolution augmented and virtual reality displays and on-chip light sources for ultra-broadband chiplet communication. However, unlike silicon scaling in electronic integrated circuits, patterning of inorganic III-V semiconductors in LEDs considerably compromises device efficiencies at submicrometer scales. Here, we present the scalable fabrication of nanoscale organic LEDs (nano-OLEDs), with the highest array density (>84,000 pixels per inch) and the smallest pixel size (~100 nm) ever reported to date. Direct nanomolecular patterning of organic semiconductors is realized by self-aligned evaporation through nanoapertures fabricated on a free-standing silicon nitride film adhering to the substrate. The average external quantum efficiencies (EQEs) extracted from a nano-OLED device of more than 4 megapixels reach up to 10%. At the subwavelength scale, individual pixels act as electroluminescent meta-atoms forming metasurfaces that directly convert electricity into modulated light. The diffractive coupling between nano-pixels enables control over the far-field emission properties, including directionality and polarization. The results presented here lay the foundation for bright surface light sources of dimension smaller than the Abbe diffraction limit, offering new technological platforms for super-resolution imaging, spectroscopy, sensing, and hybrid integrated photonics.
title Nanomolecular OLED Pixelization Enabling Electroluminescent Metasurfaces
topic Optics
Materials Science
url https://arxiv.org/abs/2404.05336