Photon bunching in high-harmonic emission controlled by quantum light

Fuente: arXiv
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Autori principali: Lemieux, Samuel, Jalil, Sohail A., Purschke, David, Boroumand, Neda, Villeneuve, David, Naumov, Andrei, Brabec, Thomas, Vampa, Giulio
Natura: Preprint
Pubblicazione: 2024
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author Lemieux, Samuel
Jalil, Sohail A.
Purschke, David
Boroumand, Neda
Villeneuve, David
Naumov, Andrei
Brabec, Thomas
Vampa, Giulio
author_facet Lemieux, Samuel
Jalil, Sohail A.
Purschke, David
Boroumand, Neda
Villeneuve, David
Naumov, Andrei
Brabec, Thomas
Vampa, Giulio
contents Attosecond spectroscopy comprises several techniques to probe matter through electrons and photons. One frontier of attosecond methods is to reveal complex phenomena arising from quantum-mechanical correlations in the matter system, in the photon fields and among them. Recent theories have laid the groundwork for understanding how quantum-optical properties affect high-field photonics, such as strong-field ionization and acceleration of electrons in quantum-optical fields, and how entanglement between the field modes arises during the interaction. Here we demonstrate a new experimental approach that transduces some properties of a quantum-optical state through a strong-field nonlinearity. We perturb high-harmonic emission from a semiconductor with a bright squeezed vacuum field resulting in the emission of sidebands of the high-harmonics with super-Poissonian statistics, indicating that the emitted photons are bunched. Our results suggest that perturbing strong-field dynamics with quantum-optical states is a viable way to coherently control the generation of these states at short wavelengths, such as extreme ultraviolet or soft X-rays. Quantum correlations will be instrumental to advance attosecond spectroscopy and imaging beyond the classical limits.
format Preprint
id arxiv_https___arxiv_org_abs_2404_05474
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Photon bunching in high-harmonic emission controlled by quantum light
Lemieux, Samuel
Jalil, Sohail A.
Purschke, David
Boroumand, Neda
Villeneuve, David
Naumov, Andrei
Brabec, Thomas
Vampa, Giulio
Quantum Physics
Optics
Attosecond spectroscopy comprises several techniques to probe matter through electrons and photons. One frontier of attosecond methods is to reveal complex phenomena arising from quantum-mechanical correlations in the matter system, in the photon fields and among them. Recent theories have laid the groundwork for understanding how quantum-optical properties affect high-field photonics, such as strong-field ionization and acceleration of electrons in quantum-optical fields, and how entanglement between the field modes arises during the interaction. Here we demonstrate a new experimental approach that transduces some properties of a quantum-optical state through a strong-field nonlinearity. We perturb high-harmonic emission from a semiconductor with a bright squeezed vacuum field resulting in the emission of sidebands of the high-harmonics with super-Poissonian statistics, indicating that the emitted photons are bunched. Our results suggest that perturbing strong-field dynamics with quantum-optical states is a viable way to coherently control the generation of these states at short wavelengths, such as extreme ultraviolet or soft X-rays. Quantum correlations will be instrumental to advance attosecond spectroscopy and imaging beyond the classical limits.
title Photon bunching in high-harmonic emission controlled by quantum light
topic Quantum Physics
Optics
url https://arxiv.org/abs/2404.05474