Spin conductances and magnetization production in chiral molecular junctions

Fuente: arXiv
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Autores principales: Korytár, Richard, van Ruitenbeek, Jan M., Evers, Ferdinand
Formato: Preprint
Publicado: 2024
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author Korytár, Richard
van Ruitenbeek, Jan M.
Evers, Ferdinand
author_facet Korytár, Richard
van Ruitenbeek, Jan M.
Evers, Ferdinand
contents Motivated by experimental reports on chirality induced spin selectivity, we investigate a minimal model that allows us to calculate the charge and spin conductances through helical molecules analytically. The spin-orbit interaction is assumed to be non-vanishing on the molecule and negligible in the reservoirs (leads). The band-structure of the molecule features four helical modes with spin-momentum locking that are analogous of edge-currents in the quantum spin Hall effect. While charge is conserved and therefore the charge current is independent of where it is measured, - reservoirs or molecule, - our detailed calculations reveal that the spin currents in the left and right lead are equal in magnitudes but with opposite signs (in linear response). We predict that transport currents flowing through helical molecules are accompanied by a spin accumulation in the contact region with the same magnetization direction for source and drain. Further, we predict that the spin-conductance can be extracted directly from measuring the (quasi-static) spin accumulation - rather than the spin current itself, which is very challenging to obtain experimentally.
format Preprint
id arxiv_https___arxiv_org_abs_2404_05614
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Spin conductances and magnetization production in chiral molecular junctions
Korytár, Richard
van Ruitenbeek, Jan M.
Evers, Ferdinand
Mesoscale and Nanoscale Physics
Motivated by experimental reports on chirality induced spin selectivity, we investigate a minimal model that allows us to calculate the charge and spin conductances through helical molecules analytically. The spin-orbit interaction is assumed to be non-vanishing on the molecule and negligible in the reservoirs (leads). The band-structure of the molecule features four helical modes with spin-momentum locking that are analogous of edge-currents in the quantum spin Hall effect. While charge is conserved and therefore the charge current is independent of where it is measured, - reservoirs or molecule, - our detailed calculations reveal that the spin currents in the left and right lead are equal in magnitudes but with opposite signs (in linear response). We predict that transport currents flowing through helical molecules are accompanied by a spin accumulation in the contact region with the same magnetization direction for source and drain. Further, we predict that the spin-conductance can be extracted directly from measuring the (quasi-static) spin accumulation - rather than the spin current itself, which is very challenging to obtain experimentally.
title Spin conductances and magnetization production in chiral molecular junctions
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2404.05614