Highly spin-polarized molecules via collisional microwave pumping

Fuente: arXiv
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Autori principali: Hermsmeier, Rebekah, Tscherbul, Timur V.
Natura: Preprint
Pubblicazione: 2024
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author Hermsmeier, Rebekah
Tscherbul, Timur V.
author_facet Hermsmeier, Rebekah
Tscherbul, Timur V.
contents We propose a general technique to produce cold spin-polarized molecules, in which rotationally excited states are first populated by coherent microwave excitation, and then allowed to spin-flip and relax via collisional quenching, which populates a single final spin state. We illustrate the high selectivity of the technique for $^{13}$C$^{16}$O molecules immersed in a cold buffer gas of helium atoms, achieving a high degree ($\geq$95\%) of nuclear spin polarization at 1 K.
format Preprint
id arxiv_https___arxiv_org_abs_2404_07416
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Highly spin-polarized molecules via collisional microwave pumping
Hermsmeier, Rebekah
Tscherbul, Timur V.
Chemical Physics
Atomic Physics
Quantum Physics
We propose a general technique to produce cold spin-polarized molecules, in which rotationally excited states are first populated by coherent microwave excitation, and then allowed to spin-flip and relax via collisional quenching, which populates a single final spin state. We illustrate the high selectivity of the technique for $^{13}$C$^{16}$O molecules immersed in a cold buffer gas of helium atoms, achieving a high degree ($\geq$95\%) of nuclear spin polarization at 1 K.
title Highly spin-polarized molecules via collisional microwave pumping
topic Chemical Physics
Atomic Physics
Quantum Physics
url https://arxiv.org/abs/2404.07416