Superpolarized Electron-Hole Liquid and Multiferroicity in Multilayer Graphene

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Autori principali: Das, Mainak, Huang, Chunli
Natura: Preprint
Pubblicazione: 2024
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author Das, Mainak
Huang, Chunli
author_facet Das, Mainak
Huang, Chunli
contents We introduce a many-body state termed superpolarized electron-hole liquid to explain the multiferroic properties observed in a recent experiment on rhombohedral pentalayer graphene by Han et al. [Nature 623, 41-47, 2023] . Superpolarization refers to a state where electrons and holes are fully polarized in opposite directions within the extended spin-valley space, resulting in a polarization per charge that exceeds the saturated value of one. This state exhibits multiferroic order, characterized by spontaneous spin, layer, and valley polarization. We demonstrate the independent control of valley polarization and orbital magnetization in this state through the application of electric-displacement field and weak magnetic fields. The large magnetoelectric effect observed in the experiment is attributed to the substantial Berry curvature concentrated near the band edge. The concept of superpolarization can be probed experimentally through magnetic oscillation and local current distribution measurements to determine the area of the Fermi surfaces and their magnetic moments.
format Preprint
id arxiv_https___arxiv_org_abs_2404_10069
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Superpolarized Electron-Hole Liquid and Multiferroicity in Multilayer Graphene
Das, Mainak
Huang, Chunli
Mesoscale and Nanoscale Physics
Materials Science
We introduce a many-body state termed superpolarized electron-hole liquid to explain the multiferroic properties observed in a recent experiment on rhombohedral pentalayer graphene by Han et al. [Nature 623, 41-47, 2023] . Superpolarization refers to a state where electrons and holes are fully polarized in opposite directions within the extended spin-valley space, resulting in a polarization per charge that exceeds the saturated value of one. This state exhibits multiferroic order, characterized by spontaneous spin, layer, and valley polarization. We demonstrate the independent control of valley polarization and orbital magnetization in this state through the application of electric-displacement field and weak magnetic fields. The large magnetoelectric effect observed in the experiment is attributed to the substantial Berry curvature concentrated near the band edge. The concept of superpolarization can be probed experimentally through magnetic oscillation and local current distribution measurements to determine the area of the Fermi surfaces and their magnetic moments.
title Superpolarized Electron-Hole Liquid and Multiferroicity in Multilayer Graphene
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2404.10069