Laser excitation of the $^{229}$Th nuclear isomeric transition in a solid-state host

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Hauptverfasser: Elwell, R., Schneider, Christian, Jeet, Justin, Terhune, J. E. S., Morgan, H. W. T., Alexandrova, A. N., Tan, H. B. Tran, Derevianko, Andrei, Hudson, Eric R.
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Veröffentlicht: 2024
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author Elwell, R.
Schneider, Christian
Jeet, Justin
Terhune, J. E. S.
Morgan, H. W. T.
Alexandrova, A. N.
Tan, H. B. Tran
Derevianko, Andrei
Hudson, Eric R.
author_facet Elwell, R.
Schneider, Christian
Jeet, Justin
Terhune, J. E. S.
Morgan, H. W. T.
Alexandrova, A. N.
Tan, H. B. Tran
Derevianko, Andrei
Hudson, Eric R.
contents LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that produces red-shifted fluorescence that decays with a timescale of a few seconds. The second is a narrow, laser-linewidth-limited spectral feature at $148.38219(4)_{\textrm{stat}}(20)_{\textrm{sys}}$ nm ($2020407.3(5)_{\textrm{stat}}(30)_{\textrm{sys}}$ GHz) that decays with a lifetime of $568(13)_{\textrm{stat}}(20)_{\textrm{sys}}$ s. This feature is assigned to the excitation of the $^{229}$Th nuclear isomeric state, whose energy is found to be $8.355733(2)_{\textrm{stat}}(10)_{\textrm{sys}}$ eV in $^{229}$Th:\thor:LiSrAlF$_6$.
format Preprint
id arxiv_https___arxiv_org_abs_2404_12311
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Laser excitation of the $^{229}$Th nuclear isomeric transition in a solid-state host
Elwell, R.
Schneider, Christian
Jeet, Justin
Terhune, J. E. S.
Morgan, H. W. T.
Alexandrova, A. N.
Tan, H. B. Tran
Derevianko, Andrei
Hudson, Eric R.
Atomic Physics
Nuclear Experiment
LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that produces red-shifted fluorescence that decays with a timescale of a few seconds. The second is a narrow, laser-linewidth-limited spectral feature at $148.38219(4)_{\textrm{stat}}(20)_{\textrm{sys}}$ nm ($2020407.3(5)_{\textrm{stat}}(30)_{\textrm{sys}}$ GHz) that decays with a lifetime of $568(13)_{\textrm{stat}}(20)_{\textrm{sys}}$ s. This feature is assigned to the excitation of the $^{229}$Th nuclear isomeric state, whose energy is found to be $8.355733(2)_{\textrm{stat}}(10)_{\textrm{sys}}$ eV in $^{229}$Th:\thor:LiSrAlF$_6$.
title Laser excitation of the $^{229}$Th nuclear isomeric transition in a solid-state host
topic Atomic Physics
Nuclear Experiment
url https://arxiv.org/abs/2404.12311