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Main Authors: Wang, Yuxin, Zheng, Zhiyue, Zhang, Qiuxin, Lai, Yonglang, Ge, Zongqi, Wang, Tianyi, Ding, Liangyu, Vasilii, Smirnov, Semerikov, Ilya, Zhang, Shuaining, Zhang, Wei, Zhang, Xiang
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2404.14734
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author Wang, Yuxin
Zheng, Zhiyue
Zhang, Qiuxin
Lai, Yonglang
Ge, Zongqi
Wang, Tianyi
Ding, Liangyu
Vasilii, Smirnov
Semerikov, Ilya
Zhang, Shuaining
Zhang, Wei
Zhang, Xiang
author_facet Wang, Yuxin
Zheng, Zhiyue
Zhang, Qiuxin
Lai, Yonglang
Ge, Zongqi
Wang, Tianyi
Ding, Liangyu
Vasilii, Smirnov
Semerikov, Ilya
Zhang, Shuaining
Zhang, Wei
Zhang, Xiang
contents We propose a novel pulsed optical field method that alternately switches the pump beam in conventional saturation absorption to time-division multiplex the same probe beam into both probe and reference beams, followed by digital differential processing to achieve deterministic zero-background Doppler-free spectroscopy. This method effectively mitigates Doppler broadening and common-mode optical noise by addressing disturbances such as non-uniform background absorption and environmental noise, thereby offering enhanced accuracy and robustness. Using this technique, we measured the absolute frequency of Yb$^{+}$ isotopes in the $6s^2\ ^{1}S_0\to 6s6p ^{1}P_1$ transition. By employing an error signal derived from the first-derivative demodulated spectrum of $^{174}\mathrm{Yb}^{+}$, we achieved efficient stabilization of a 369.5 nm ultraviolet diode laser, demonstrating a frequency stability of $3 \times 10^{-11}$ over a 1500-second averaging period and a locking point uncertainty of 850 kHz sustained over 10 days. Furthermore, we report the first in-situ observation of Doppler-free Zeeman sub-level spectra, highlighting the precision of this method and its potential application in measuring magnetic field gradients.
format Preprint
id arxiv_https___arxiv_org_abs_2404_14734
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle In-situ Doppler-free spectroscopy with pulsed optical fields
Wang, Yuxin
Zheng, Zhiyue
Zhang, Qiuxin
Lai, Yonglang
Ge, Zongqi
Wang, Tianyi
Ding, Liangyu
Vasilii, Smirnov
Semerikov, Ilya
Zhang, Shuaining
Zhang, Wei
Zhang, Xiang
Optics
We propose a novel pulsed optical field method that alternately switches the pump beam in conventional saturation absorption to time-division multiplex the same probe beam into both probe and reference beams, followed by digital differential processing to achieve deterministic zero-background Doppler-free spectroscopy. This method effectively mitigates Doppler broadening and common-mode optical noise by addressing disturbances such as non-uniform background absorption and environmental noise, thereby offering enhanced accuracy and robustness. Using this technique, we measured the absolute frequency of Yb$^{+}$ isotopes in the $6s^2\ ^{1}S_0\to 6s6p ^{1}P_1$ transition. By employing an error signal derived from the first-derivative demodulated spectrum of $^{174}\mathrm{Yb}^{+}$, we achieved efficient stabilization of a 369.5 nm ultraviolet diode laser, demonstrating a frequency stability of $3 \times 10^{-11}$ over a 1500-second averaging period and a locking point uncertainty of 850 kHz sustained over 10 days. Furthermore, we report the first in-situ observation of Doppler-free Zeeman sub-level spectra, highlighting the precision of this method and its potential application in measuring magnetic field gradients.
title In-situ Doppler-free spectroscopy with pulsed optical fields
topic Optics
url https://arxiv.org/abs/2404.14734