Towards electrical domain-wall control in polyacetylene-based electronic nanodevices

Fuente: arXiv
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Main Authors: Arancibia, Leandro M., Bertoni, Andrés I., Sánchez, Cristián G., Lobos, Alejandro M.
Format: Preprint
Published: 2024
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author Arancibia, Leandro M.
Bertoni, Andrés I.
Sánchez, Cristián G.
Lobos, Alejandro M.
author_facet Arancibia, Leandro M.
Bertoni, Andrés I.
Sánchez, Cristián G.
Lobos, Alejandro M.
contents We theoretically propose a polymer-based nano-device consisting of a single trans-polyacetylene (tPA) molecule capacitively coupled to external voltage gates. We model the integrated device using a Su-Schrieffer-Heeger (SSH)-like Hamiltonian, and we demonstrate the emergence of localized domain walls (DWs) with quantized charges (i.e., soliton excitations) localized at the gates. Interestingly, by increasing the applied voltage, multiple discrete charges can be accumulated, which may be useful for potential technological applications. Exploiting the topological character of the solitonic excitations of tPA, this device can be considered as an organic-based quantum dot with a very large and robust quantized charge.
format Preprint
id arxiv_https___arxiv_org_abs_2404_15257
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Towards electrical domain-wall control in polyacetylene-based electronic nanodevices
Arancibia, Leandro M.
Bertoni, Andrés I.
Sánchez, Cristián G.
Lobos, Alejandro M.
Mesoscale and Nanoscale Physics
We theoretically propose a polymer-based nano-device consisting of a single trans-polyacetylene (tPA) molecule capacitively coupled to external voltage gates. We model the integrated device using a Su-Schrieffer-Heeger (SSH)-like Hamiltonian, and we demonstrate the emergence of localized domain walls (DWs) with quantized charges (i.e., soliton excitations) localized at the gates. Interestingly, by increasing the applied voltage, multiple discrete charges can be accumulated, which may be useful for potential technological applications. Exploiting the topological character of the solitonic excitations of tPA, this device can be considered as an organic-based quantum dot with a very large and robust quantized charge.
title Towards electrical domain-wall control in polyacetylene-based electronic nanodevices
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2404.15257