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Bibliographic Details
Main Authors: Gauthier, Alexandre, Sobota, Jonathan A., Gauthier, Nicolas, Rotundu, Costel R., Shen, Zhi-Xun, Kirchmann, Patrick S.
Format: Preprint
Published: 2024
Subjects:
Online Access:https://arxiv.org/abs/2404.17203
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Table of Contents:
  • Bi$_2$Se$_3$ has been the focus of intense interest over the past decade due to its topological properties. Bi surfaces are known to form on Bi$_2$Se$_3$ upon exposure to atmosphere, but their electronic structure has not been investigated. We report band structure measurements of such Bi surfaces using angle-resolved photoemission spectroscopy. Measured spectra can be well explained by the band structure of a single bilayer of Bi on Bi$_2$Se$_3$, and show that Bi surfaces consistently dominate the photoemission signal for air exposure times of at least 1 hour. These results demonstrate that atmospheric effects should be taken into consideration when identifying two-dimensional transport channels, and when designing surface-sensitive measurements of Bi$_2$Se$_3$, ideally limiting air exposure to no more than a few minutes.