Disruptive Forces in Metamaterial Tweezers for Trapping 20 nm Nanoparticles Based on Molecular Graphene Quantum Dots

Fuente: arXiv
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Auteurs principaux: Bouloumis, Theodoros D., Zhao, Hao, Kokkinidis, Nikolaos, Hu, Yunbin, Truong, Viet Giang, Narita, Akimitsu, Chormaic, Síle Nic
Format: Preprint
Publié: 2024
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author Bouloumis, Theodoros D.
Zhao, Hao
Kokkinidis, Nikolaos
Hu, Yunbin
Truong, Viet Giang
Narita, Akimitsu
Chormaic, Síle Nic
author_facet Bouloumis, Theodoros D.
Zhao, Hao
Kokkinidis, Nikolaos
Hu, Yunbin
Truong, Viet Giang
Narita, Akimitsu
Chormaic, Síle Nic
contents In recent years, plasmonic optical tweezers have been used to trap nanoparticles and study interactions with their environment. An unavoidable challenge is the plasmonic heating due to resonant excitation and the resulting temperature rise in the surrounding environment. In this work, we demonstrate trapping of custom-synthesized 20 nm nanoparticles based on molecular graphene quantum dots using metamaterial plasmonic tweezers. Superior trap stiffness values as high as 8.8 (fN/nm)/(mW/$μ\mbox{m}^2$) were achieved with optical intensities lower than 1 mW/$μ\mbox{m}^2$. By gradually increasing the laser intensity we identified a critical value beyond which the stiffness values dropped significantly. This value corresponded to a temperature rise of about 16$^o$C, evidently sufficient to create thermal flows and disrupt the trapping performance. We, therefore, identified a safe intensity regime for trapping nanoparticles without unwanted heat. Our platform can be used for efficient nanopositioning of fluorescent particles and quantum emitters in an array configuration, potentially acting as a single-photon source configuration.
format Preprint
id arxiv_https___arxiv_org_abs_2404_17307
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Disruptive Forces in Metamaterial Tweezers for Trapping 20 nm Nanoparticles Based on Molecular Graphene Quantum Dots
Bouloumis, Theodoros D.
Zhao, Hao
Kokkinidis, Nikolaos
Hu, Yunbin
Truong, Viet Giang
Narita, Akimitsu
Chormaic, Síle Nic
Optics
Applied Physics
In recent years, plasmonic optical tweezers have been used to trap nanoparticles and study interactions with their environment. An unavoidable challenge is the plasmonic heating due to resonant excitation and the resulting temperature rise in the surrounding environment. In this work, we demonstrate trapping of custom-synthesized 20 nm nanoparticles based on molecular graphene quantum dots using metamaterial plasmonic tweezers. Superior trap stiffness values as high as 8.8 (fN/nm)/(mW/$μ\mbox{m}^2$) were achieved with optical intensities lower than 1 mW/$μ\mbox{m}^2$. By gradually increasing the laser intensity we identified a critical value beyond which the stiffness values dropped significantly. This value corresponded to a temperature rise of about 16$^o$C, evidently sufficient to create thermal flows and disrupt the trapping performance. We, therefore, identified a safe intensity regime for trapping nanoparticles without unwanted heat. Our platform can be used for efficient nanopositioning of fluorescent particles and quantum emitters in an array configuration, potentially acting as a single-photon source configuration.
title Disruptive Forces in Metamaterial Tweezers for Trapping 20 nm Nanoparticles Based on Molecular Graphene Quantum Dots
topic Optics
Applied Physics
url https://arxiv.org/abs/2404.17307