Ferroelectricity in twisted double bilayer graphene

Fuente: arXiv
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Autori principali: Du, Renjun, Xiao, Jingkuan, Zhang, Di, Cai, Xiaofan, Jiang, Siqi, Lian, Fuzhuo, Watanabe, Kenji, Taniguchi, Takashi, Wang, Lei, Yu, Geliang
Natura: Preprint
Pubblicazione: 2024
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author Du, Renjun
Xiao, Jingkuan
Zhang, Di
Cai, Xiaofan
Jiang, Siqi
Lian, Fuzhuo
Watanabe, Kenji
Taniguchi, Takashi
Wang, Lei
Yu, Geliang
author_facet Du, Renjun
Xiao, Jingkuan
Zhang, Di
Cai, Xiaofan
Jiang, Siqi
Lian, Fuzhuo
Watanabe, Kenji
Taniguchi, Takashi
Wang, Lei
Yu, Geliang
contents Two-dimensional ferroelectrics can maintain vertical polarization up to room temperature, and are, therefore, promising for next-generation nonvolatile memories. Although natural two-dimensional ferroelectrics are few, moiré superlattices provide us with a generalized method to construct ferroelectrics from non-ferroelectric parent materials. We report a realization of ferroelectric hysteresis in a AB-BA stacked twisted double bilayer graphene (TDBG) system. The ferroelectric polarization is prominent at zero external displacement field and reduces upon increasing displacement fields. TDBG in the AB-BA configuration possesses a superlattice of non-centrosymmetric domains, exhibiting alternatively switchable polarities even without the assistance of any boron nitride layers; however, in the AB-AB stacking case, the development of polarized domains necessitates the presence of a second superlattice induced by the adjacent boron nitride layer. Therefore, twisted multilayer graphene systems offer us a fascinating field to explore two-dimensional ferroelectricity.
format Preprint
id arxiv_https___arxiv_org_abs_2404_18059
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Ferroelectricity in twisted double bilayer graphene
Du, Renjun
Xiao, Jingkuan
Zhang, Di
Cai, Xiaofan
Jiang, Siqi
Lian, Fuzhuo
Watanabe, Kenji
Taniguchi, Takashi
Wang, Lei
Yu, Geliang
Mesoscale and Nanoscale Physics
Two-dimensional ferroelectrics can maintain vertical polarization up to room temperature, and are, therefore, promising for next-generation nonvolatile memories. Although natural two-dimensional ferroelectrics are few, moiré superlattices provide us with a generalized method to construct ferroelectrics from non-ferroelectric parent materials. We report a realization of ferroelectric hysteresis in a AB-BA stacked twisted double bilayer graphene (TDBG) system. The ferroelectric polarization is prominent at zero external displacement field and reduces upon increasing displacement fields. TDBG in the AB-BA configuration possesses a superlattice of non-centrosymmetric domains, exhibiting alternatively switchable polarities even without the assistance of any boron nitride layers; however, in the AB-AB stacking case, the development of polarized domains necessitates the presence of a second superlattice induced by the adjacent boron nitride layer. Therefore, twisted multilayer graphene systems offer us a fascinating field to explore two-dimensional ferroelectricity.
title Ferroelectricity in twisted double bilayer graphene
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2404.18059