Realization of a Two-Dimensional Lieb Lattice in a Metal-Inorganic Framework with Flat Bands and Topological Edge States

Fuente: arXiv
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Main Authors: Wu, Wenjun, Sun, Shuo, Tang, Chi Sin, Wu, Jing, Ma, Yu, Zhang, Lingfeng, Cai, Chuanbing, Zhong, Jianxin, Milošević, Milorad V., Wee, Andrew T. S., Yin, Xinmao
Format: Preprint
Published: 2024
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author Wu, Wenjun
Sun, Shuo
Tang, Chi Sin
Wu, Jing
Ma, Yu
Zhang, Lingfeng
Cai, Chuanbing
Zhong, Jianxin
Milošević, Milorad V.
Wee, Andrew T. S.
Yin, Xinmao
author_facet Wu, Wenjun
Sun, Shuo
Tang, Chi Sin
Wu, Jing
Ma, Yu
Zhang, Lingfeng
Cai, Chuanbing
Zhong, Jianxin
Milošević, Milorad V.
Wee, Andrew T. S.
Yin, Xinmao
contents Flat bands and Dirac cones in materials are at the source of the exotic electronic and topological properties. The Lieb lattice is expected to host these electronic structures, arising from quantum destructive interference. Nevertheless, the experimental realization of a two-dimensional Lieb lattice remained challenging to date due to its intrinsic structural instability. After computationally designing a Platinum-Phosphorus (Pt-P) Lieb lattice, we have successfully overcome its structural instability and synthesized it on a gold substrate via molecular beam epitaxy. Low-temperature scanning tunneling microscopy and spectroscopy verified the Lieb lattice's morphology and electronic flat bands. Furthermore, topological Dirac edge states stemming from pronounced spin-orbit coupling induced by heavy Pt atoms have been predicted. These findings convincingly open perspectives for creating metal-inorganic framework-based atomic lattices, offering prospects for strongly correlated phases interplayed with topology.
format Preprint
id arxiv_https___arxiv_org_abs_2404_18430
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Realization of a Two-Dimensional Lieb Lattice in a Metal-Inorganic Framework with Flat Bands and Topological Edge States
Wu, Wenjun
Sun, Shuo
Tang, Chi Sin
Wu, Jing
Ma, Yu
Zhang, Lingfeng
Cai, Chuanbing
Zhong, Jianxin
Milošević, Milorad V.
Wee, Andrew T. S.
Yin, Xinmao
Applied Physics
Materials Science
Flat bands and Dirac cones in materials are at the source of the exotic electronic and topological properties. The Lieb lattice is expected to host these electronic structures, arising from quantum destructive interference. Nevertheless, the experimental realization of a two-dimensional Lieb lattice remained challenging to date due to its intrinsic structural instability. After computationally designing a Platinum-Phosphorus (Pt-P) Lieb lattice, we have successfully overcome its structural instability and synthesized it on a gold substrate via molecular beam epitaxy. Low-temperature scanning tunneling microscopy and spectroscopy verified the Lieb lattice's morphology and electronic flat bands. Furthermore, topological Dirac edge states stemming from pronounced spin-orbit coupling induced by heavy Pt atoms have been predicted. These findings convincingly open perspectives for creating metal-inorganic framework-based atomic lattices, offering prospects for strongly correlated phases interplayed with topology.
title Realization of a Two-Dimensional Lieb Lattice in a Metal-Inorganic Framework with Flat Bands and Topological Edge States
topic Applied Physics
Materials Science
url https://arxiv.org/abs/2404.18430