Composite antiferromagnetic and orbital order with altermagnetic properties at a cuprate/manganite interface

Fuente: arXiv
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Hauptverfasser: Sarkar, Subhrangsu, Capu, Roxana, Pashkevich, Yurii G., Knobel, Jonas, Cantarino, Marli R., Nag, Abhishek, Kummer, Kurt, Betto, Davide, Sant, Roberto, Nicholson, Christopher W., Khmaladze, Jarji, Zhou, Ke-jin., Brookes, Nicholas B., Monney, Claude, Bernhard, Christian
Format: Preprint
Veröffentlicht: 2024
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author Sarkar, Subhrangsu
Capu, Roxana
Pashkevich, Yurii G.
Knobel, Jonas
Cantarino, Marli R.
Nag, Abhishek
Kummer, Kurt
Betto, Davide
Sant, Roberto
Nicholson, Christopher W.
Khmaladze, Jarji
Zhou, Ke-jin.
Brookes, Nicholas B.
Monney, Claude
Bernhard, Christian
author_facet Sarkar, Subhrangsu
Capu, Roxana
Pashkevich, Yurii G.
Knobel, Jonas
Cantarino, Marli R.
Nag, Abhishek
Kummer, Kurt
Betto, Davide
Sant, Roberto
Nicholson, Christopher W.
Khmaladze, Jarji
Zhou, Ke-jin.
Brookes, Nicholas B.
Monney, Claude
Bernhard, Christian
contents Heterostructures from complex oxides allow one to combine various electronic and magnetic orders as to induce new quantum states. A prominent example is the coupling between superconducting and magnetic orders in multilayers from high-Tc cuprates and manganites. A key role is played here by the interfacial CuO2 layer whose distinct properties remain to be fully understood. Here, we study with resonant inelastic X-ray scattering (RIXS) the magnon excitations of this interfacial CuO2 layer. In particular, we show that the underlying antiferromagnetic exchange interaction at the interface is strongly suppressed to J ~ 70 meV, as compared to J ~ 130 meV for the CuO2 layers away from the interface. Moreover, we observe an anomalous momentum dependence of the intensity of the interfacial magnon mode and show that it suggests that the antiferromagnetic order is accompanied by a particular kind of orbital order that yields a so-called altermagnetic state. Such a two-dimensional altermagnet has recently been predicted to enable new spintronic applications and superconducting proximity effects.
format Preprint
id arxiv_https___arxiv_org_abs_2404_19410
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Composite antiferromagnetic and orbital order with altermagnetic properties at a cuprate/manganite interface
Sarkar, Subhrangsu
Capu, Roxana
Pashkevich, Yurii G.
Knobel, Jonas
Cantarino, Marli R.
Nag, Abhishek
Kummer, Kurt
Betto, Davide
Sant, Roberto
Nicholson, Christopher W.
Khmaladze, Jarji
Zhou, Ke-jin.
Brookes, Nicholas B.
Monney, Claude
Bernhard, Christian
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
Superconductivity
Heterostructures from complex oxides allow one to combine various electronic and magnetic orders as to induce new quantum states. A prominent example is the coupling between superconducting and magnetic orders in multilayers from high-Tc cuprates and manganites. A key role is played here by the interfacial CuO2 layer whose distinct properties remain to be fully understood. Here, we study with resonant inelastic X-ray scattering (RIXS) the magnon excitations of this interfacial CuO2 layer. In particular, we show that the underlying antiferromagnetic exchange interaction at the interface is strongly suppressed to J ~ 70 meV, as compared to J ~ 130 meV for the CuO2 layers away from the interface. Moreover, we observe an anomalous momentum dependence of the intensity of the interfacial magnon mode and show that it suggests that the antiferromagnetic order is accompanied by a particular kind of orbital order that yields a so-called altermagnetic state. Such a two-dimensional altermagnet has recently been predicted to enable new spintronic applications and superconducting proximity effects.
title Composite antiferromagnetic and orbital order with altermagnetic properties at a cuprate/manganite interface
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
Superconductivity
url https://arxiv.org/abs/2404.19410