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Main Authors: Dey, Urmimala, McCabe, Emma E., Íñiguez-González, Jorge, Bristowe, Nicholas C.
Format: Preprint
Published: 2024
Subjects:
Online Access:https://arxiv.org/abs/2405.01307
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author Dey, Urmimala
McCabe, Emma E.
Íñiguez-González, Jorge
Bristowe, Nicholas C.
author_facet Dey, Urmimala
McCabe, Emma E.
Íñiguez-González, Jorge
Bristowe, Nicholas C.
contents The promise of a strong magnetoelectric coupling in a multiferroic material is not only of fundamental interest, but also forms the basis of next generation memory devices where the direction of magnetization can be reversed by an external electric field. Using group-theory led first-principles calculations, we have identified a hitherto unknown polar phase of the $A_4B_3\rm{O}_9$ layered oxides, where the polar mode couples to the magnetic modes through a rare $Γ$-point magnetoelectric-multiferroic coupling scheme such that the net magnetization can be directly reversed by an electric field switching of the polar mode. Furthermore, in agreement with previous experimental observations, we predict room temperature magnetism in $A_4B_3\rm{O}_9$ oxides which indicates the promising practical applications of these compounds in the next generation memory devices.
format Preprint
id arxiv_https___arxiv_org_abs_2405_01307
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Prediction of Room Temperature Electric Field Reversal of Magnetization in the Family of $A_4B_3\rm{O}_9$ Layered Oxides
Dey, Urmimala
McCabe, Emma E.
Íñiguez-González, Jorge
Bristowe, Nicholas C.
Materials Science
The promise of a strong magnetoelectric coupling in a multiferroic material is not only of fundamental interest, but also forms the basis of next generation memory devices where the direction of magnetization can be reversed by an external electric field. Using group-theory led first-principles calculations, we have identified a hitherto unknown polar phase of the $A_4B_3\rm{O}_9$ layered oxides, where the polar mode couples to the magnetic modes through a rare $Γ$-point magnetoelectric-multiferroic coupling scheme such that the net magnetization can be directly reversed by an electric field switching of the polar mode. Furthermore, in agreement with previous experimental observations, we predict room temperature magnetism in $A_4B_3\rm{O}_9$ oxides which indicates the promising practical applications of these compounds in the next generation memory devices.
title Prediction of Room Temperature Electric Field Reversal of Magnetization in the Family of $A_4B_3\rm{O}_9$ Layered Oxides
topic Materials Science
url https://arxiv.org/abs/2405.01307