Bayesian uncertainty quantification for synthesizing superheavy elements

Fuente: arXiv
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Auteurs principaux: Fang, Yueping, Gao, Zepeng, Zhang, Yinu, Liao, Zehong, Yang, Yu, Su, Jun, Zhu, Long
Format: Preprint
Publié: 2024
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author Fang, Yueping
Gao, Zepeng
Zhang, Yinu
Liao, Zehong
Yang, Yu
Su, Jun
Zhu, Long
author_facet Fang, Yueping
Gao, Zepeng
Zhang, Yinu
Liao, Zehong
Yang, Yu
Su, Jun
Zhu, Long
contents To improve the theoretical prediction power for synthesizing superheavy elements beyond Og, a Bayesian uncertainty quantification method is employed to evaluate the uncertainty of the calculated evaporation residue cross sections (ERCS) for the first time. The key parameters of the dinuclear system (DNS) model, such as the diffusion parameter $\textit{a}$, the damping factor $E_\mathrm{d}$, and the level-density parameter ratio $a_\mathrm{f}/a_\mathrm{n}$ are systematically constrained by the Bayesian analysis of recent ERCS data. One intriguing behavior is shown that the optimal incident energies (OIE) corresponding to the largest ERCS weakly depend on the fission process. We also find that these parameters are strongly correlated and the uncertainty propagation considering the parameters independently is not reasonable. The 2$σ$ confidence level of posterior distributions for $a = 0.586_{-0.002}^{+0.002}$ fm, $E_\mathrm{d} = 25.65_{-3.41}^{+3.43}$ MeV, and $a_\mathrm{f}/a_\mathrm{n} = 1.081_{-0.021}^{+0.021}$ are obtained. Furthermore, the confidence levels of the ERCS and OIE for synthesizing Z = 119 via the reactions($^{54}\mathrm{Cr}+^{243}\mathrm{Am}$), (${}^{50}\mathrm{Ti}+{}^{249}\mathrm{Bk}$), and (${}^{51}\mathrm{V}+{}^{248}\mathrm{Cm}$) are predicted. This work sets the stage for future analyses to explore the OIE and reaction systems for the synthesis of superheavy elements.
format Preprint
id arxiv_https___arxiv_org_abs_2405_02839
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Bayesian uncertainty quantification for synthesizing superheavy elements
Fang, Yueping
Gao, Zepeng
Zhang, Yinu
Liao, Zehong
Yang, Yu
Su, Jun
Zhu, Long
Nuclear Theory
To improve the theoretical prediction power for synthesizing superheavy elements beyond Og, a Bayesian uncertainty quantification method is employed to evaluate the uncertainty of the calculated evaporation residue cross sections (ERCS) for the first time. The key parameters of the dinuclear system (DNS) model, such as the diffusion parameter $\textit{a}$, the damping factor $E_\mathrm{d}$, and the level-density parameter ratio $a_\mathrm{f}/a_\mathrm{n}$ are systematically constrained by the Bayesian analysis of recent ERCS data. One intriguing behavior is shown that the optimal incident energies (OIE) corresponding to the largest ERCS weakly depend on the fission process. We also find that these parameters are strongly correlated and the uncertainty propagation considering the parameters independently is not reasonable. The 2$σ$ confidence level of posterior distributions for $a = 0.586_{-0.002}^{+0.002}$ fm, $E_\mathrm{d} = 25.65_{-3.41}^{+3.43}$ MeV, and $a_\mathrm{f}/a_\mathrm{n} = 1.081_{-0.021}^{+0.021}$ are obtained. Furthermore, the confidence levels of the ERCS and OIE for synthesizing Z = 119 via the reactions($^{54}\mathrm{Cr}+^{243}\mathrm{Am}$), (${}^{50}\mathrm{Ti}+{}^{249}\mathrm{Bk}$), and (${}^{51}\mathrm{V}+{}^{248}\mathrm{Cm}$) are predicted. This work sets the stage for future analyses to explore the OIE and reaction systems for the synthesis of superheavy elements.
title Bayesian uncertainty quantification for synthesizing superheavy elements
topic Nuclear Theory
url https://arxiv.org/abs/2405.02839