Observation of Mermin-Wagner behavior in LaFeO$_3$/SrTiO$_3$ superlattices

Fuente: arXiv
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Autori principali: Kiaba, Michal, Suter, Andreas, Salman, Zaher, Prokscha, Thomas, Chen, Binbin, Koster, Gertjan, Dubroka, Adam
Natura: Preprint
Pubblicazione: 2024
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author Kiaba, Michal
Suter, Andreas
Salman, Zaher
Prokscha, Thomas
Chen, Binbin
Koster, Gertjan
Dubroka, Adam
author_facet Kiaba, Michal
Suter, Andreas
Salman, Zaher
Prokscha, Thomas
Chen, Binbin
Koster, Gertjan
Dubroka, Adam
contents Two-dimensional magnetic materials attract a lot of attention since they potentially exhibit new magnetic properties due to, e.g., strongly enhanced spin fluctuations. However, the suppression of the long-range magnetic order in two dimensions due to long-wavelength spin fluctuations, as suggested by the Mermin-Wagner theorem, has been questioned for finite-size laboratory samples. Here we study the magnetic properties of a dimensional crossover in superlattices composed of the antiferromagnetic LaFeO$_3$ and SrTiO$_3$ that, thanks to their large lateral size, allowed examination using a sensitive magnetic probe - muon spin rotation spectroscopy. We show that the iron electronic moments in superlattices with 3 and 2 monolayers of LaFeO$_3$ exhibit a static antiferromagnetic order. In contrast, in the superlattices with single LaFeO$_3$ monolayer, the moments do not order and fluctuate to the lowest measured temperature as expected from the Mermin-Wagner theorem. Our work shows how dimensionality can be used to tune the magnetic properties of ultrathin films.
format Preprint
id arxiv_https___arxiv_org_abs_2405_04293
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Observation of Mermin-Wagner behavior in LaFeO$_3$/SrTiO$_3$ superlattices
Kiaba, Michal
Suter, Andreas
Salman, Zaher
Prokscha, Thomas
Chen, Binbin
Koster, Gertjan
Dubroka, Adam
Strongly Correlated Electrons
Materials Science
Two-dimensional magnetic materials attract a lot of attention since they potentially exhibit new magnetic properties due to, e.g., strongly enhanced spin fluctuations. However, the suppression of the long-range magnetic order in two dimensions due to long-wavelength spin fluctuations, as suggested by the Mermin-Wagner theorem, has been questioned for finite-size laboratory samples. Here we study the magnetic properties of a dimensional crossover in superlattices composed of the antiferromagnetic LaFeO$_3$ and SrTiO$_3$ that, thanks to their large lateral size, allowed examination using a sensitive magnetic probe - muon spin rotation spectroscopy. We show that the iron electronic moments in superlattices with 3 and 2 monolayers of LaFeO$_3$ exhibit a static antiferromagnetic order. In contrast, in the superlattices with single LaFeO$_3$ monolayer, the moments do not order and fluctuate to the lowest measured temperature as expected from the Mermin-Wagner theorem. Our work shows how dimensionality can be used to tune the magnetic properties of ultrathin films.
title Observation of Mermin-Wagner behavior in LaFeO$_3$/SrTiO$_3$ superlattices
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2405.04293