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Main Authors: Huang, Hanshen, Qu, Tao, Cheng, Yang, Tai, Lixuan, Eckberg, Christopher, Pan, Quanjun, Alrasheed, Abdullah, Chong, Su Kong, Dai, Bingqian, Li, Yaochen, Shu, Qingyuan, Yang, Chao-Yao, Yu, Jie-Xiang, Yin, Gen, Wang, Kang L.
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2405.04686
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author Huang, Hanshen
Qu, Tao
Cheng, Yang
Tai, Lixuan
Eckberg, Christopher
Pan, Quanjun
Alrasheed, Abdullah
Chong, Su Kong
Dai, Bingqian
Li, Yaochen
Shu, Qingyuan
Yang, Chao-Yao
Yu, Jie-Xiang
Yin, Gen
Wang, Kang L.
author_facet Huang, Hanshen
Qu, Tao
Cheng, Yang
Tai, Lixuan
Eckberg, Christopher
Pan, Quanjun
Alrasheed, Abdullah
Chong, Su Kong
Dai, Bingqian
Li, Yaochen
Shu, Qingyuan
Yang, Chao-Yao
Yu, Jie-Xiang
Yin, Gen
Wang, Kang L.
contents Antiferromagnet is a promising candidate for the next generation spintronic devices, benefiting from its ultrafast dynamics and spontaneous zero stray field. However, the understanding of their ultrafast spin behaviors is lacking due to the challenges of controlling/detecting the quenched net magnetization. Unconventional compensated semiconducting antiferromagnets present strong time-reversal symmetry breaking, spin splitting in the momentum space, and suitable bandgap for optical control/detection. Thus, it is a powerful platform to uncover the ultrafast dynamics of antiferromagnets. Here, we show an exotic wavelength-dependent spin dynamic in the unconventional compensated semiconducting antiferromagnet α-MnTe via time-resolved quadratic magneto-optical Kerr effect measurement, where the probing photon energy of the laser matches its bandgap. This direct excitation and detection of distinct magnon modes reveal varying spin behaviors and time characteristics in a broad temperature range. It originates from the spins triggered at different bands of electronic structures and is depicted in an energy transfer model among electrons, phonons, and magnons. Our study of exotic optical properties in this unconventional semiconducting antiferromagnet fulfills the missing information of spin evolution in the time domain and paves the way for its utilization in ultrafast spintronic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2405_04686
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Ultrafast dynamics of wavelength-sensitive magnons in unconventional compensated semiconducting antiferromagnet
Huang, Hanshen
Qu, Tao
Cheng, Yang
Tai, Lixuan
Eckberg, Christopher
Pan, Quanjun
Alrasheed, Abdullah
Chong, Su Kong
Dai, Bingqian
Li, Yaochen
Shu, Qingyuan
Yang, Chao-Yao
Yu, Jie-Xiang
Yin, Gen
Wang, Kang L.
Applied Physics
Optics
Antiferromagnet is a promising candidate for the next generation spintronic devices, benefiting from its ultrafast dynamics and spontaneous zero stray field. However, the understanding of their ultrafast spin behaviors is lacking due to the challenges of controlling/detecting the quenched net magnetization. Unconventional compensated semiconducting antiferromagnets present strong time-reversal symmetry breaking, spin splitting in the momentum space, and suitable bandgap for optical control/detection. Thus, it is a powerful platform to uncover the ultrafast dynamics of antiferromagnets. Here, we show an exotic wavelength-dependent spin dynamic in the unconventional compensated semiconducting antiferromagnet α-MnTe via time-resolved quadratic magneto-optical Kerr effect measurement, where the probing photon energy of the laser matches its bandgap. This direct excitation and detection of distinct magnon modes reveal varying spin behaviors and time characteristics in a broad temperature range. It originates from the spins triggered at different bands of electronic structures and is depicted in an energy transfer model among electrons, phonons, and magnons. Our study of exotic optical properties in this unconventional semiconducting antiferromagnet fulfills the missing information of spin evolution in the time domain and paves the way for its utilization in ultrafast spintronic devices.
title Ultrafast dynamics of wavelength-sensitive magnons in unconventional compensated semiconducting antiferromagnet
topic Applied Physics
Optics
url https://arxiv.org/abs/2405.04686