Controlled molecule injector for cold, dense, and pure molecular beams at the European x-ray free-electron laser

Fuente: arXiv
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Auteurs principaux: He, Lanhai, Johny, Melby, Kierspel, Thomas, Długołęcki, Karol, Bari, Sadia, Boll, Rebecca, Bromberger, Hubertus, Coreno, Marcello, De Fanis, Alberto, Di Fraia, Michele, Erk, Benjamin, Gisselbrecht, Mathieu, Grychtol, Patrik, Eng-Johnsson, Per, Mazza, Tommaso, Onvlee, Jolijn, Ovcharenko, Yevheniy, Petrovic, Jovana, Rennhack, Nils, Rivas, Daniel E., Rudenko, Artem, Rühl, Eckart, Schwob, Lucas, Simon, Marc, Trinter, Florian, Usenko, Sergey, Wiese, Joss, Meyer, Michael, Trippel, Sebastian, Küpper, Jochen
Format: Preprint
Publié: 2024
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author He, Lanhai
Johny, Melby
Kierspel, Thomas
Długołęcki, Karol
Bari, Sadia
Boll, Rebecca
Bromberger, Hubertus
Coreno, Marcello
De Fanis, Alberto
Di Fraia, Michele
Erk, Benjamin
Gisselbrecht, Mathieu
Grychtol, Patrik
Eng-Johnsson, Per
Mazza, Tommaso
Onvlee, Jolijn
Ovcharenko, Yevheniy
Petrovic, Jovana
Rennhack, Nils
Rivas, Daniel E.
Rudenko, Artem
Rühl, Eckart
Schwob, Lucas
Simon, Marc
Trinter, Florian
Usenko, Sergey
Wiese, Joss
Meyer, Michael
Trippel, Sebastian
Küpper, Jochen
author_facet He, Lanhai
Johny, Melby
Kierspel, Thomas
Długołęcki, Karol
Bari, Sadia
Boll, Rebecca
Bromberger, Hubertus
Coreno, Marcello
De Fanis, Alberto
Di Fraia, Michele
Erk, Benjamin
Gisselbrecht, Mathieu
Grychtol, Patrik
Eng-Johnsson, Per
Mazza, Tommaso
Onvlee, Jolijn
Ovcharenko, Yevheniy
Petrovic, Jovana
Rennhack, Nils
Rivas, Daniel E.
Rudenko, Artem
Rühl, Eckart
Schwob, Lucas
Simon, Marc
Trinter, Florian
Usenko, Sergey
Wiese, Joss
Meyer, Michael
Trippel, Sebastian
Küpper, Jochen
contents A permanently available molecular-beam injection setup for controlled molecules (COMO) was installed and commissioned at the small quantum systems (SQS) instrument at the European x-ray free-electron laser (EuXFEL). A $b$-type electrostatic deflector allows for pure state-, size-, and isomer-selected samples of polar molecules and clusters. The source provides a rotationally cold ($T\approx1$~K) and dense ($ρ\approx10^8$~cm$^{-3}$) molecular beam with pulse durations up to 100~\us generated by a new version of the Even-Lavie valve. Here, a performance overview of the COMO setup is presented along with characterization experiments performed both, with an optical laser at the Center for Free-Electron-Laser Science and with x-rays at EuXFEL under burst-mode operation. COMO was designed to be attached to different instruments at the EuXFEL, in particular at the small quantum systems (SQS) and single particles, clusters, and biomolecules (SPB) instruments. This advanced controlled-molecules injection setup enables XFEL studies using highly defined samples with soft and hard x-ray FEL radiation for applications ranging from atomic, molecular, and cluster physics to elementary processes in chemistry and biology.
format Preprint
id arxiv_https___arxiv_org_abs_2405_06344
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Controlled molecule injector for cold, dense, and pure molecular beams at the European x-ray free-electron laser
He, Lanhai
Johny, Melby
Kierspel, Thomas
Długołęcki, Karol
Bari, Sadia
Boll, Rebecca
Bromberger, Hubertus
Coreno, Marcello
De Fanis, Alberto
Di Fraia, Michele
Erk, Benjamin
Gisselbrecht, Mathieu
Grychtol, Patrik
Eng-Johnsson, Per
Mazza, Tommaso
Onvlee, Jolijn
Ovcharenko, Yevheniy
Petrovic, Jovana
Rennhack, Nils
Rivas, Daniel E.
Rudenko, Artem
Rühl, Eckart
Schwob, Lucas
Simon, Marc
Trinter, Florian
Usenko, Sergey
Wiese, Joss
Meyer, Michael
Trippel, Sebastian
Küpper, Jochen
Chemical Physics
Atomic and Molecular Clusters
A permanently available molecular-beam injection setup for controlled molecules (COMO) was installed and commissioned at the small quantum systems (SQS) instrument at the European x-ray free-electron laser (EuXFEL). A $b$-type electrostatic deflector allows for pure state-, size-, and isomer-selected samples of polar molecules and clusters. The source provides a rotationally cold ($T\approx1$~K) and dense ($ρ\approx10^8$~cm$^{-3}$) molecular beam with pulse durations up to 100~\us generated by a new version of the Even-Lavie valve. Here, a performance overview of the COMO setup is presented along with characterization experiments performed both, with an optical laser at the Center for Free-Electron-Laser Science and with x-rays at EuXFEL under burst-mode operation. COMO was designed to be attached to different instruments at the EuXFEL, in particular at the small quantum systems (SQS) and single particles, clusters, and biomolecules (SPB) instruments. This advanced controlled-molecules injection setup enables XFEL studies using highly defined samples with soft and hard x-ray FEL radiation for applications ranging from atomic, molecular, and cluster physics to elementary processes in chemistry and biology.
title Controlled molecule injector for cold, dense, and pure molecular beams at the European x-ray free-electron laser
topic Chemical Physics
Atomic and Molecular Clusters
url https://arxiv.org/abs/2405.06344