Unveiling the Pockels Coefficient of Ferroelectric Nitride ScAlN

Fuente: arXiv
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Autori principali: Yang, Guangcanlan, Wang, Haochen, Mu, Sai, Xie, Hao, Wang, Tyler, He, Chengxing, Shen, Mohan, Liu, Mengxia, Van de Walle, Chris G., Tang, Hong X.
Natura: Preprint
Pubblicazione: 2024
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author Yang, Guangcanlan
Wang, Haochen
Mu, Sai
Xie, Hao
Wang, Tyler
He, Chengxing
Shen, Mohan
Liu, Mengxia
Van de Walle, Chris G.
Tang, Hong X.
author_facet Yang, Guangcanlan
Wang, Haochen
Mu, Sai
Xie, Hao
Wang, Tyler
He, Chengxing
Shen, Mohan
Liu, Mengxia
Van de Walle, Chris G.
Tang, Hong X.
contents Nitride ferroelectrics have recently emerged as promising alternatives to oxide ferroelectrics due to their compatibility with mainstream semiconductor processing. ScAlN, in particular, has exhibited remarkable piezoelectric coupling strength ($K^2$) comparable to that of lithium niobate (LN), making it a valuable choice for RF filters in wireless communications. Recently, ScAlN has sparked interest in its use for nanophotonic devices, chiefly due to its large bandgap facilitating operation in blue wavelengths coupled with promises of enhanced nonlinear optical properties such as a large second-order susceptibility ($χ^{(2)}$). It is still an open question whether ScAlN can outperform oxide ferroelectrics concerning the Pockels effect -- an electro-optic coupling extensively utilized in optical communications devices. In this paper, we present a comprehensive theoretical analysis and experimental demonstration of ScAlN's Pockels effect. Our findings reveal that the electro-optic coupling of ScAlN, despite being weak at low Sc concentration, may be significantly enhanced and exceed LiNbO$_3$ at high levels of Sc doping, which points the direction of continued research efforts to unlock the full potential of ScAlN.
format Preprint
id arxiv_https___arxiv_org_abs_2405_07978
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Unveiling the Pockels Coefficient of Ferroelectric Nitride ScAlN
Yang, Guangcanlan
Wang, Haochen
Mu, Sai
Xie, Hao
Wang, Tyler
He, Chengxing
Shen, Mohan
Liu, Mengxia
Van de Walle, Chris G.
Tang, Hong X.
Materials Science
Applied Physics
Optics
Nitride ferroelectrics have recently emerged as promising alternatives to oxide ferroelectrics due to their compatibility with mainstream semiconductor processing. ScAlN, in particular, has exhibited remarkable piezoelectric coupling strength ($K^2$) comparable to that of lithium niobate (LN), making it a valuable choice for RF filters in wireless communications. Recently, ScAlN has sparked interest in its use for nanophotonic devices, chiefly due to its large bandgap facilitating operation in blue wavelengths coupled with promises of enhanced nonlinear optical properties such as a large second-order susceptibility ($χ^{(2)}$). It is still an open question whether ScAlN can outperform oxide ferroelectrics concerning the Pockels effect -- an electro-optic coupling extensively utilized in optical communications devices. In this paper, we present a comprehensive theoretical analysis and experimental demonstration of ScAlN's Pockels effect. Our findings reveal that the electro-optic coupling of ScAlN, despite being weak at low Sc concentration, may be significantly enhanced and exceed LiNbO$_3$ at high levels of Sc doping, which points the direction of continued research efforts to unlock the full potential of ScAlN.
title Unveiling the Pockels Coefficient of Ferroelectric Nitride ScAlN
topic Materials Science
Applied Physics
Optics
url https://arxiv.org/abs/2405.07978