The Flux Hypothesis for Odd Transport Phenomena

Fuente: arXiv
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Autori principali: Hargus, Cory, Deshpande, Alhad, Omar, Ahmad K., Mandadapu, Kranthi K.
Natura: Preprint
Pubblicazione: 2024
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author Hargus, Cory
Deshpande, Alhad
Omar, Ahmad K.
Mandadapu, Kranthi K.
author_facet Hargus, Cory
Deshpande, Alhad
Omar, Ahmad K.
Mandadapu, Kranthi K.
contents Onsager's regression hypothesis makes a fundamental connection between macroscopic transport phenomena and the average relaxation of spontaneous microscopic fluctuations. This relaxation, however, is agnostic to odd transport phenomena, in which fluxes run orthogonal to the gradients driving them. To account for odd transport, we generalize the regression hypothesis, postulating that macroscopic linear constitutive laws are, on average, obeyed by microscopic fluctuations, whether they contribute to relaxation or not. From this "flux hypothesis," Green-Kubo and reciprocal relations follow, elucidating the separate roles of broken time-reversal and parity symmetries underlying various odd transport coefficients. As an application, we derive and verify the Green-Kubo relation for odd collective diffusion in chiral active matter, first in an analytically-tractable model and subsequently through molecular dynamics simulations of concentrated active spinners.
format Preprint
id arxiv_https___arxiv_org_abs_2405_08798
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle The Flux Hypothesis for Odd Transport Phenomena
Hargus, Cory
Deshpande, Alhad
Omar, Ahmad K.
Mandadapu, Kranthi K.
Statistical Mechanics
Soft Condensed Matter
Chemical Physics
Onsager's regression hypothesis makes a fundamental connection between macroscopic transport phenomena and the average relaxation of spontaneous microscopic fluctuations. This relaxation, however, is agnostic to odd transport phenomena, in which fluxes run orthogonal to the gradients driving them. To account for odd transport, we generalize the regression hypothesis, postulating that macroscopic linear constitutive laws are, on average, obeyed by microscopic fluctuations, whether they contribute to relaxation or not. From this "flux hypothesis," Green-Kubo and reciprocal relations follow, elucidating the separate roles of broken time-reversal and parity symmetries underlying various odd transport coefficients. As an application, we derive and verify the Green-Kubo relation for odd collective diffusion in chiral active matter, first in an analytically-tractable model and subsequently through molecular dynamics simulations of concentrated active spinners.
title The Flux Hypothesis for Odd Transport Phenomena
topic Statistical Mechanics
Soft Condensed Matter
Chemical Physics
url https://arxiv.org/abs/2405.08798