1/3 and other magnetization plateaus in a quasi-one-dimensional Ising magnet $\mathbf{TbTi_3Bi_4}$ with zigzag spin chain

Fuente: arXiv
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Auteurs principaux: Guo, Kaizhen, Ma, Zeyu, Liu, Hongxiong, Wu, Ziyang, Wang, Junfeng, Shi, Youguo, Li, Yuan, Jia, Shuang
Format: Preprint
Publié: 2024
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author Guo, Kaizhen
Ma, Zeyu
Liu, Hongxiong
Wu, Ziyang
Wang, Junfeng
Shi, Youguo
Li, Yuan
Jia, Shuang
author_facet Guo, Kaizhen
Ma, Zeyu
Liu, Hongxiong
Wu, Ziyang
Wang, Junfeng
Shi, Youguo
Li, Yuan
Jia, Shuang
contents We report the magnetic properties of newly synthesized, single crystals of $\mathrm{TbTi_3Bi_4}$ whose crystal structure is highlighted by the stacking of terbium-based zigzag chains and titanium-based kagome lattices. This compound demonstrates extreme easy-axis magnetic anisotropy due to the crystalline-electric-field effect which aligns the $\mathrm{Tb^{3+}}$ moments along the zigzag chain direction. As the result of the strong single-ion anisotropy and multiple magnetic interactions, $\mathrm{TbTi_3Bi_4}$ behaves as a quasi-one-dimensional Ising magnet with a remarkable antiferromagnetic ordering at $T_\mathrm{N}$ = 20.4 K. When a magnetic field is applied along the direction of the zigzag chain, multiple meta-magnetic transitions occur between 1/3 and other magnetization plateaus. We have created a field-temperature phase diagram and mapped out the complex magnetic structures resulting from frustration.
format Preprint
id arxiv_https___arxiv_org_abs_2405_09280
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle 1/3 and other magnetization plateaus in a quasi-one-dimensional Ising magnet $\mathbf{TbTi_3Bi_4}$ with zigzag spin chain
Guo, Kaizhen
Ma, Zeyu
Liu, Hongxiong
Wu, Ziyang
Wang, Junfeng
Shi, Youguo
Li, Yuan
Jia, Shuang
Strongly Correlated Electrons
We report the magnetic properties of newly synthesized, single crystals of $\mathrm{TbTi_3Bi_4}$ whose crystal structure is highlighted by the stacking of terbium-based zigzag chains and titanium-based kagome lattices. This compound demonstrates extreme easy-axis magnetic anisotropy due to the crystalline-electric-field effect which aligns the $\mathrm{Tb^{3+}}$ moments along the zigzag chain direction. As the result of the strong single-ion anisotropy and multiple magnetic interactions, $\mathrm{TbTi_3Bi_4}$ behaves as a quasi-one-dimensional Ising magnet with a remarkable antiferromagnetic ordering at $T_\mathrm{N}$ = 20.4 K. When a magnetic field is applied along the direction of the zigzag chain, multiple meta-magnetic transitions occur between 1/3 and other magnetization plateaus. We have created a field-temperature phase diagram and mapped out the complex magnetic structures resulting from frustration.
title 1/3 and other magnetization plateaus in a quasi-one-dimensional Ising magnet $\mathbf{TbTi_3Bi_4}$ with zigzag spin chain
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2405.09280