Determination of the Néel vector in rutile altermagnets through x-ray magnetic circular dichroism: the case of MnF$_2$

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Main Authors: Hariki, A., Okauchi, T., Takahashi, Y., Kuneš, J.
Format: Preprint
Published: 2024
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_version_ 1866909307178582016
author Hariki, A.
Okauchi, T.
Takahashi, Y.
Kuneš, J.
author_facet Hariki, A.
Okauchi, T.
Takahashi, Y.
Kuneš, J.
contents We present a numerical simulation of the X-ray magnetic circular dichroism (XMCD) at the $L_{2,3}$ edge of Mn in altermagnetic MnF$_2$ using a combination of density functional + exact diagonlization of an atomic model. We explore how the dichroic spectra vary with the light propagation vector and the Néel vector. We show how XMCD in rutile structures can be employed to determine the orientation of the Néel vector. An exact relationship between the XMCD spectra for different orientation of the Néel vector valid in the absence on the valence spin-orbit coupling and core-valence multipole interaction is derived and its approximate validity demonstrated by numerical calculation for the full Hamiltonian.
format Preprint
id arxiv_https___arxiv_org_abs_2405_11833
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Determination of the Néel vector in rutile altermagnets through x-ray magnetic circular dichroism: the case of MnF$_2$
Hariki, A.
Okauchi, T.
Takahashi, Y.
Kuneš, J.
Strongly Correlated Electrons
Materials Science
We present a numerical simulation of the X-ray magnetic circular dichroism (XMCD) at the $L_{2,3}$ edge of Mn in altermagnetic MnF$_2$ using a combination of density functional + exact diagonlization of an atomic model. We explore how the dichroic spectra vary with the light propagation vector and the Néel vector. We show how XMCD in rutile structures can be employed to determine the orientation of the Néel vector. An exact relationship between the XMCD spectra for different orientation of the Néel vector valid in the absence on the valence spin-orbit coupling and core-valence multipole interaction is derived and its approximate validity demonstrated by numerical calculation for the full Hamiltonian.
title Determination of the Néel vector in rutile altermagnets through x-ray magnetic circular dichroism: the case of MnF$_2$
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2405.11833