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Main Authors: Kaplan, Daniel, Volkov, Pavel A., Chakraborty, Ahana, Zhuang, Zekun, Chandra, Premala
Format: Preprint
Published: 2024
Subjects:
Online Access:https://arxiv.org/abs/2405.12214
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author Kaplan, Daniel
Volkov, Pavel A.
Chakraborty, Ahana
Zhuang, Zekun
Chandra, Premala
author_facet Kaplan, Daniel
Volkov, Pavel A.
Chakraborty, Ahana
Zhuang, Zekun
Chandra, Premala
contents We show that driving optical phonons above a threshold fluence induces spatiotemporal orders, where material properties oscillate at an incommensurate wavevector $q_0$ in space and at half the drive frequency in time. The order is robust against temperature on timescales much larger than the lifetime of the excited modes and can be accompanied by a static $2q_0$ modulation. We make predictions for time-resolved diffraction and provide estimates for candidate materials. Our results show the possibility of using THz waves in solids to realize tunable incommensurate order on the nanoscale.
format Preprint
id arxiv_https___arxiv_org_abs_2405_12214
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Tunable Spatiotemporal Orders in Driven Insulators
Kaplan, Daniel
Volkov, Pavel A.
Chakraborty, Ahana
Zhuang, Zekun
Chandra, Premala
Mesoscale and Nanoscale Physics
Materials Science
Statistical Mechanics
We show that driving optical phonons above a threshold fluence induces spatiotemporal orders, where material properties oscillate at an incommensurate wavevector $q_0$ in space and at half the drive frequency in time. The order is robust against temperature on timescales much larger than the lifetime of the excited modes and can be accompanied by a static $2q_0$ modulation. We make predictions for time-resolved diffraction and provide estimates for candidate materials. Our results show the possibility of using THz waves in solids to realize tunable incommensurate order on the nanoscale.
title Tunable Spatiotemporal Orders in Driven Insulators
topic Mesoscale and Nanoscale Physics
Materials Science
Statistical Mechanics
url https://arxiv.org/abs/2405.12214