Nano-gap electrode dielectrophoresis for tether-free trapping and interferometric-scattering detection of single 20 nm particles

Fuente: arXiv
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Main Authors: Ton, Jacco, Travers, Théo, Soltani, Jamal, Wijnperle, Daniel, Shavlovskyi, Dmytro, Orrit, Michel, Pud, Sergii
Format: Preprint
Published: 2024
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author Ton, Jacco
Travers, Théo
Soltani, Jamal
Wijnperle, Daniel
Shavlovskyi, Dmytro
Orrit, Michel
Pud, Sergii
author_facet Ton, Jacco
Travers, Théo
Soltani, Jamal
Wijnperle, Daniel
Shavlovskyi, Dmytro
Orrit, Michel
Pud, Sergii
contents Accurate detection and characterization of nanoparticles within confined spaces is crucial for applications ranging from nanofluidics to biotechnology. We present a novel approach that combines interferometric scattering (iSCAT) detection with trapping by dielectrophoresis (DEP) to achieve label-free detection of nanoparticles that are trapped and/or actuated between nano-gap electrodes. DEP utilizes the interaction between the induced dipole of the particle and the applied electric field to create a trapping potential. We demonstrate our method by trapping and label-free detection of down to 20 nm polystyrene nanoparticles. Additionally, we demonstrate that the signal-to-noise ratio of our detection can be boosted up to 20-fold by periodic actuation of the nanoparticle in the trap. This is done by a digital lock-in detection scheme on the modulated scattering signal. Our method holds promise for various applications, including assembly of nanoparticles, single-particle property analysis, and nanofluidic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2405_12338
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Nano-gap electrode dielectrophoresis for tether-free trapping and interferometric-scattering detection of single 20 nm particles
Ton, Jacco
Travers, Théo
Soltani, Jamal
Wijnperle, Daniel
Shavlovskyi, Dmytro
Orrit, Michel
Pud, Sergii
Optics
Chemical Physics
Accurate detection and characterization of nanoparticles within confined spaces is crucial for applications ranging from nanofluidics to biotechnology. We present a novel approach that combines interferometric scattering (iSCAT) detection with trapping by dielectrophoresis (DEP) to achieve label-free detection of nanoparticles that are trapped and/or actuated between nano-gap electrodes. DEP utilizes the interaction between the induced dipole of the particle and the applied electric field to create a trapping potential. We demonstrate our method by trapping and label-free detection of down to 20 nm polystyrene nanoparticles. Additionally, we demonstrate that the signal-to-noise ratio of our detection can be boosted up to 20-fold by periodic actuation of the nanoparticle in the trap. This is done by a digital lock-in detection scheme on the modulated scattering signal. Our method holds promise for various applications, including assembly of nanoparticles, single-particle property analysis, and nanofluidic devices.
title Nano-gap electrode dielectrophoresis for tether-free trapping and interferometric-scattering detection of single 20 nm particles
topic Optics
Chemical Physics
url https://arxiv.org/abs/2405.12338