Three-dimensional mapping of the altermagnetic spin splitting in CrSb

Fuente: arXiv
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Main Authors: Yang, Guowei, Li, Zhanghuan, Yang, Sai, Li, Jiyuan, Zheng, Hao, Zhu, Weifan, Pan, Ze, Xu, Yifu, Cao, Saizheng, Zhao, Wenxuan, Jana, Anupam, Zhang, Jiawen, Ye, Mao, Song, Yu, Hu, Lun-Hui, Yang, Lexian, Fujii, Jun, Vobornik, Ivana, Shi, Ming, Yuan, Huiqiu, Zhang, Yongjun, Xu, Yuanfeng, Liu, Yang
Format: Preprint
Published: 2024
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author Yang, Guowei
Li, Zhanghuan
Yang, Sai
Li, Jiyuan
Zheng, Hao
Zhu, Weifan
Pan, Ze
Xu, Yifu
Cao, Saizheng
Zhao, Wenxuan
Jana, Anupam
Zhang, Jiawen
Ye, Mao
Song, Yu
Hu, Lun-Hui
Yang, Lexian
Fujii, Jun
Vobornik, Ivana
Shi, Ming
Yuan, Huiqiu
Zhang, Yongjun
Xu, Yuanfeng
Liu, Yang
author_facet Yang, Guowei
Li, Zhanghuan
Yang, Sai
Li, Jiyuan
Zheng, Hao
Zhu, Weifan
Pan, Ze
Xu, Yifu
Cao, Saizheng
Zhao, Wenxuan
Jana, Anupam
Zhang, Jiawen
Ye, Mao
Song, Yu
Hu, Lun-Hui
Yang, Lexian
Fujii, Jun
Vobornik, Ivana
Shi, Ming
Yuan, Huiqiu
Zhang, Yongjun
Xu, Yuanfeng
Liu, Yang
contents Altermagnetism, a kind of collinear magnetism that is characterized by a momentum-dependent band and spin splitting without net magnetization, has recently attracted considerable interest. Finding altermagnetic materials with large splitting near the Fermi level necessarily requires three-dimensional k-space mapping. While this is crucial for spintronic applications and emergent phenomena, it remains challenging. Here, using synchrotron-based angle-resolved photoemission spectroscopy (ARPES), spin-resolved ARPES and model calculations, we uncover a large altermagnetic splitting, up to ~1.0 eV, near the Fermi level in CrSb. We verify its bulk-type g-wave altermagnetism through systematic three-dimensional k-space mapping, which unambiguously reveals the altermagnetic symmetry and associated nodal planes. Spin-resolved ARPES measurements further verify the spin polarizations of the split bands near Fermi level. Tight-binding model analysis indicates that the large altermagnetic splitting arises from strong third-nearest-neighbor hopping mediated by Sb ions. The large band/spin splitting near Fermi level in metallic CrSb, together with its high TN (up to 705 K) and simple spin configuration, paves the way for exploring emergent phenomena and spintronic applications based on altermagnets.
format Preprint
id arxiv_https___arxiv_org_abs_2405_12575
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Three-dimensional mapping of the altermagnetic spin splitting in CrSb
Yang, Guowei
Li, Zhanghuan
Yang, Sai
Li, Jiyuan
Zheng, Hao
Zhu, Weifan
Pan, Ze
Xu, Yifu
Cao, Saizheng
Zhao, Wenxuan
Jana, Anupam
Zhang, Jiawen
Ye, Mao
Song, Yu
Hu, Lun-Hui
Yang, Lexian
Fujii, Jun
Vobornik, Ivana
Shi, Ming
Yuan, Huiqiu
Zhang, Yongjun
Xu, Yuanfeng
Liu, Yang
Materials Science
Strongly Correlated Electrons
Altermagnetism, a kind of collinear magnetism that is characterized by a momentum-dependent band and spin splitting without net magnetization, has recently attracted considerable interest. Finding altermagnetic materials with large splitting near the Fermi level necessarily requires three-dimensional k-space mapping. While this is crucial for spintronic applications and emergent phenomena, it remains challenging. Here, using synchrotron-based angle-resolved photoemission spectroscopy (ARPES), spin-resolved ARPES and model calculations, we uncover a large altermagnetic splitting, up to ~1.0 eV, near the Fermi level in CrSb. We verify its bulk-type g-wave altermagnetism through systematic three-dimensional k-space mapping, which unambiguously reveals the altermagnetic symmetry and associated nodal planes. Spin-resolved ARPES measurements further verify the spin polarizations of the split bands near Fermi level. Tight-binding model analysis indicates that the large altermagnetic splitting arises from strong third-nearest-neighbor hopping mediated by Sb ions. The large band/spin splitting near Fermi level in metallic CrSb, together with its high TN (up to 705 K) and simple spin configuration, paves the way for exploring emergent phenomena and spintronic applications based on altermagnets.
title Three-dimensional mapping of the altermagnetic spin splitting in CrSb
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2405.12575