Light induced magnetic order

Fuente: arXiv
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Auteurs principaux: Jauk, T., Hampel, H., Walowski, J., Komatsu, K., Kredl, J., Harris-Lee, E. I., Dewhurst, J. K., Münzenberg, M., Shallcross, S., Sharma, S., Schultze, M.
Format: Preprint
Publié: 2024
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author Jauk, T.
Hampel, H.
Walowski, J.
Komatsu, K.
Kredl, J.
Harris-Lee, E. I.
Dewhurst, J. K.
Münzenberg, M.
Shallcross, S.
Sharma, S.
Schultze, M.
author_facet Jauk, T.
Hampel, H.
Walowski, J.
Komatsu, K.
Kredl, J.
Harris-Lee, E. I.
Dewhurst, J. K.
Münzenberg, M.
Shallcross, S.
Sharma, S.
Schultze, M.
contents Heat and disorder are opponents of magnetism. This fact, expressed in Curie's law established more than a century ago, holds even in the highly non-equilibrium interaction of ultra-intense laser pulses with magnetic matter. In contradiction to this, here we demonstrate that optical excitation of a ferromagnet can abrogate the link between temperature and order and observe 100 femtosecond class laser pulses to drive a reduction in spin entropy, concomitant to an increase in spin polarization and magnetic moment persisting after relaxation back to local charge equilibrium. This both establishes disorder as an unexpected resource for magnetic control at ultrafast times and, by the provision of a purely electronic mechanism that does not involve reconfiguration of the crystal lattice, suggests a novel scheme for spin-based signal processing and information storage significantly faster than current methodology.
format Preprint
id arxiv_https___arxiv_org_abs_2405_12690
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Light induced magnetic order
Jauk, T.
Hampel, H.
Walowski, J.
Komatsu, K.
Kredl, J.
Harris-Lee, E. I.
Dewhurst, J. K.
Münzenberg, M.
Shallcross, S.
Sharma, S.
Schultze, M.
Mesoscale and Nanoscale Physics
Optics
Heat and disorder are opponents of magnetism. This fact, expressed in Curie's law established more than a century ago, holds even in the highly non-equilibrium interaction of ultra-intense laser pulses with magnetic matter. In contradiction to this, here we demonstrate that optical excitation of a ferromagnet can abrogate the link between temperature and order and observe 100 femtosecond class laser pulses to drive a reduction in spin entropy, concomitant to an increase in spin polarization and magnetic moment persisting after relaxation back to local charge equilibrium. This both establishes disorder as an unexpected resource for magnetic control at ultrafast times and, by the provision of a purely electronic mechanism that does not involve reconfiguration of the crystal lattice, suggests a novel scheme for spin-based signal processing and information storage significantly faster than current methodology.
title Light induced magnetic order
topic Mesoscale and Nanoscale Physics
Optics
url https://arxiv.org/abs/2405.12690