Why Scanning Tunneling Microscopy on Sr$_2$RuO$_4$ sometimes doesn't see the superconducting gap

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Main Authors: Valadkhani, Adrian, Profe, Jonas B., Kreisel, Andreas, Hirschfeld, P. J., Valentí, Roser
Format: Preprint
Published: 2024
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_version_ 1866915039823265792
author Valadkhani, Adrian
Profe, Jonas B.
Kreisel, Andreas
Hirschfeld, P. J.
Valentí, Roser
author_facet Valadkhani, Adrian
Profe, Jonas B.
Kreisel, Andreas
Hirschfeld, P. J.
Valentí, Roser
contents Scanning tunneling microscopy (STM) is perhaps the most promising way to detect the superconducting gap size and structure in the canonical unconventional superconductor Sr$_2$RuO$_4$ directly. However, in many cases, researchers have reported being unable to detect the gap at all in simple STM conductance measurements. Recently, an investigation of this issue on various local topographic structures on a Sr-terminated surface found that superconducting spectra appeared only in the region of small nanoscale canyons, corresponding to the removal of one RuO surface layer. Here, we analyze the electronic structure of various possible surface structures using first principles methods, and argue that bulk conditions favorable for superconductivity can be achieved when removal of the RuO layer suppresses the RuO$_4$ octahedral rotation locally. We further propose alternative terminations to the most frequently reported Sr termination where superconductivity surfaces should be observed.
format Preprint
id arxiv_https___arxiv_org_abs_2405_13106
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Why Scanning Tunneling Microscopy on Sr$_2$RuO$_4$ sometimes doesn't see the superconducting gap
Valadkhani, Adrian
Profe, Jonas B.
Kreisel, Andreas
Hirschfeld, P. J.
Valentí, Roser
Superconductivity
Materials Science
Scanning tunneling microscopy (STM) is perhaps the most promising way to detect the superconducting gap size and structure in the canonical unconventional superconductor Sr$_2$RuO$_4$ directly. However, in many cases, researchers have reported being unable to detect the gap at all in simple STM conductance measurements. Recently, an investigation of this issue on various local topographic structures on a Sr-terminated surface found that superconducting spectra appeared only in the region of small nanoscale canyons, corresponding to the removal of one RuO surface layer. Here, we analyze the electronic structure of various possible surface structures using first principles methods, and argue that bulk conditions favorable for superconductivity can be achieved when removal of the RuO layer suppresses the RuO$_4$ octahedral rotation locally. We further propose alternative terminations to the most frequently reported Sr termination where superconductivity surfaces should be observed.
title Why Scanning Tunneling Microscopy on Sr$_2$RuO$_4$ sometimes doesn't see the superconducting gap
topic Superconductivity
Materials Science
url https://arxiv.org/abs/2405.13106