Adsorption of polyelectrolytes in the presence of varying dielectric discontinuity between solution and substrate

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Main Authors: Vahid, Hossein, Scacchi, Alberto, Sammalkorpi, Maria, Ala-Nissila, Tapio
Format: Preprint
Published: 2024
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author Vahid, Hossein
Scacchi, Alberto
Sammalkorpi, Maria
Ala-Nissila, Tapio
author_facet Vahid, Hossein
Scacchi, Alberto
Sammalkorpi, Maria
Ala-Nissila, Tapio
contents We examine the interactions between polyelectrolytes (PEs) and uncharged substrates at conditions corresponding to a dielectric discontinuity between the aqueous solution and the substrate. To this end, we vary the relevant system characteristics, in particular the substrate dielectric constant $\varepsilon_{\rm s}$ under different salt conditions. We employ coarse-grained molecular dynamics simulations with rodlike PEs in salt solutions with explicit ions and implicit water solvent with dielectric constant $\varepsilon_{\rm w} = 80$. As expected, at low salt concentrations, PEs are repelled from the substrates with $\varepsilon_{\rm s} < \varepsilon_{\rm w}$ but are attracted to substrates with a high dielectric constant due to image charges. This attraction considerably weakens for high salt and multivalent counterions due to enhanced screening. Further, for monovalent salt, screening enhances adsorption for weakly charged PEs, but weakens it for strongly charged ones. Multivalent counterions, on the other hand, have little effect on weakly charged PEs, but prevent adsorption of highly charged PEs, even at low salt concentrations. We also find that correlation-induced charge inversion of a PE is enhanced close to the low dielectric constant substrates, but suppressed when the dielectric constant is high. To explore the possibility of a PE monolayer formation, we examine the interaction of a pair of like-charged PEs aligned parallel to a high dielectric constant substrate with $\varepsilon_{\rm s} = 8000$. Our main conclusion is that monolayer formation is possible only for weakly charged PEs at high salt concentrations of both monovalent and multivalent counterions. Finally, we also consider the energetics of a PE approaching the substrate perpendicular to it, in analogy to polymer translocation.
format Preprint
id arxiv_https___arxiv_org_abs_2405_13484
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Adsorption of polyelectrolytes in the presence of varying dielectric discontinuity between solution and substrate
Vahid, Hossein
Scacchi, Alberto
Sammalkorpi, Maria
Ala-Nissila, Tapio
Soft Condensed Matter
We examine the interactions between polyelectrolytes (PEs) and uncharged substrates at conditions corresponding to a dielectric discontinuity between the aqueous solution and the substrate. To this end, we vary the relevant system characteristics, in particular the substrate dielectric constant $\varepsilon_{\rm s}$ under different salt conditions. We employ coarse-grained molecular dynamics simulations with rodlike PEs in salt solutions with explicit ions and implicit water solvent with dielectric constant $\varepsilon_{\rm w} = 80$. As expected, at low salt concentrations, PEs are repelled from the substrates with $\varepsilon_{\rm s} < \varepsilon_{\rm w}$ but are attracted to substrates with a high dielectric constant due to image charges. This attraction considerably weakens for high salt and multivalent counterions due to enhanced screening. Further, for monovalent salt, screening enhances adsorption for weakly charged PEs, but weakens it for strongly charged ones. Multivalent counterions, on the other hand, have little effect on weakly charged PEs, but prevent adsorption of highly charged PEs, even at low salt concentrations. We also find that correlation-induced charge inversion of a PE is enhanced close to the low dielectric constant substrates, but suppressed when the dielectric constant is high. To explore the possibility of a PE monolayer formation, we examine the interaction of a pair of like-charged PEs aligned parallel to a high dielectric constant substrate with $\varepsilon_{\rm s} = 8000$. Our main conclusion is that monolayer formation is possible only for weakly charged PEs at high salt concentrations of both monovalent and multivalent counterions. Finally, we also consider the energetics of a PE approaching the substrate perpendicular to it, in analogy to polymer translocation.
title Adsorption of polyelectrolytes in the presence of varying dielectric discontinuity between solution and substrate
topic Soft Condensed Matter
url https://arxiv.org/abs/2405.13484