Large-Scale Epitaxial Integration of Single-Crystalline BiSb Topological Insulator on GaAs (111)A

Fuente: arXiv
Gespeichert in:
Bibliographische Detailangaben
Hauptverfasser: Khaled, Mohamed Ali, Cancellara, Leonardo, Fekraoui, Salima, Daubriac, Richard, Bertran, François, Bigi, Chiara, Gravelier, Quentin, Monflier, Richard, Arnoult, Alexandre, Durand, Corentin, Plissard, Sébastien
Format: Preprint
Veröffentlicht: 2024
Schlagworte:
Online-Zugang:
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
_version_ 1866911885008306176
author Khaled, Mohamed Ali
Cancellara, Leonardo
Fekraoui, Salima
Daubriac, Richard
Bertran, François
Bigi, Chiara
Gravelier, Quentin
Monflier, Richard
Arnoult, Alexandre
Durand, Corentin
Plissard, Sébastien
author_facet Khaled, Mohamed Ali
Cancellara, Leonardo
Fekraoui, Salima
Daubriac, Richard
Bertran, François
Bigi, Chiara
Gravelier, Quentin
Monflier, Richard
Arnoult, Alexandre
Durand, Corentin
Plissard, Sébastien
contents Topological insulators (TI) are promising materials for future spintronics applications and their epitaxial integration would allow the realization of new hybrid interfaces. As the first materials studied, Bismuth Antimony alloys (Bi1-xSbx) show great potential due to their tuneable electronic band structure and efficient charge-to-spin conversion. Here, we report the growth of Bi1-xSbx thin films on GaAs (111)A substrates following two different protocols. For the conventional epitaxy process, the grown films show excellent crystallinity and twin domains corresponding to an in-plane 180{\textdegree} rotation of the crystalline structure. Domain walls are found to be composition-dependent and have a lower density for Antimony-rich films. For the optimized process, depositing an Antimony bilayer prior to BiSb growth allows achieving single crystallinity of the TI films. The topologically protected surface states are evidenced by ex-situ ARPES measurements for domains-free and conventional films. To the best of our knowledge, this work presents the first large-scale epitaxial integration of single crystalline Bi1-xSbx thin films on industrial substrates.
format Preprint
id arxiv_https___arxiv_org_abs_2405_14450
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Large-Scale Epitaxial Integration of Single-Crystalline BiSb Topological Insulator on GaAs (111)A
Khaled, Mohamed Ali
Cancellara, Leonardo
Fekraoui, Salima
Daubriac, Richard
Bertran, François
Bigi, Chiara
Gravelier, Quentin
Monflier, Richard
Arnoult, Alexandre
Durand, Corentin
Plissard, Sébastien
Materials Science
Topological insulators (TI) are promising materials for future spintronics applications and their epitaxial integration would allow the realization of new hybrid interfaces. As the first materials studied, Bismuth Antimony alloys (Bi1-xSbx) show great potential due to their tuneable electronic band structure and efficient charge-to-spin conversion. Here, we report the growth of Bi1-xSbx thin films on GaAs (111)A substrates following two different protocols. For the conventional epitaxy process, the grown films show excellent crystallinity and twin domains corresponding to an in-plane 180{\textdegree} rotation of the crystalline structure. Domain walls are found to be composition-dependent and have a lower density for Antimony-rich films. For the optimized process, depositing an Antimony bilayer prior to BiSb growth allows achieving single crystallinity of the TI films. The topologically protected surface states are evidenced by ex-situ ARPES measurements for domains-free and conventional films. To the best of our knowledge, this work presents the first large-scale epitaxial integration of single crystalline Bi1-xSbx thin films on industrial substrates.
title Large-Scale Epitaxial Integration of Single-Crystalline BiSb Topological Insulator on GaAs (111)A
topic Materials Science
url https://arxiv.org/abs/2405.14450