Extended Kohler's scaling, a low temperature anomaly and Isosbestic point in the charge density wave state of 1T-VSe$_2$

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Main Authors: Sonika, Gangwar, Sunil, Kumar, Pankaj, Taraphder, A., Yadav, C. S.
Format: Preprint
Published: 2024
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author Sonika
Gangwar, Sunil
Kumar, Pankaj
Taraphder, A.
Yadav, C. S.
author_facet Sonika
Gangwar, Sunil
Kumar, Pankaj
Taraphder, A.
Yadav, C. S.
contents 1T-VSe$_2$ is a narrow band transition metal chalcogenide that shows charge density wave (CDW) state below $T_{CDW}$ = 110 K. Here, we have explored the relevance of Kohler's rule and the thermal transport properties of VSe$_2$ across the CDW state. The magnetoresistance (MR) follows Kohler's rule above $T_{CDW}$, while an extended Kohler's rule is employed below $T_{CDW}$. Interestingly, we observed an anomaly in MR at T = 20 K, below which MR value decreases on lowering temperature. This anomaly is also reflected in the slope ($κ$) of Kohler's plots and the relative change in the thermal excitation induced carrier density ($n_T$) also. The $T_{CDW}$ remains largely unaffected in both electrical resistivity ($ρ(T)$) and longitudinal Seebeck coefficient ($\it{S_{xx}}$) even under a strong magnetic field of 14 Tesla. However, the application of magnetic field enhances the peak intensity of $\it{S_{xx}}$ at T $\sim$ 60 K. Additionally, $\it{S_{xx}(T)}$ curves measured at different fields exhibit a crossover at T = 20 K, which suggest the existence of unique feature in the CDW state of VSe$_2$ \textit{i.e.} a locally exact isosbestic point.
format Preprint
id arxiv_https___arxiv_org_abs_2405_15483
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Extended Kohler's scaling, a low temperature anomaly and Isosbestic point in the charge density wave state of 1T-VSe$_2$
Sonika
Gangwar, Sunil
Kumar, Pankaj
Taraphder, A.
Yadav, C. S.
Strongly Correlated Electrons
Materials Science
1T-VSe$_2$ is a narrow band transition metal chalcogenide that shows charge density wave (CDW) state below $T_{CDW}$ = 110 K. Here, we have explored the relevance of Kohler's rule and the thermal transport properties of VSe$_2$ across the CDW state. The magnetoresistance (MR) follows Kohler's rule above $T_{CDW}$, while an extended Kohler's rule is employed below $T_{CDW}$. Interestingly, we observed an anomaly in MR at T = 20 K, below which MR value decreases on lowering temperature. This anomaly is also reflected in the slope ($κ$) of Kohler's plots and the relative change in the thermal excitation induced carrier density ($n_T$) also. The $T_{CDW}$ remains largely unaffected in both electrical resistivity ($ρ(T)$) and longitudinal Seebeck coefficient ($\it{S_{xx}}$) even under a strong magnetic field of 14 Tesla. However, the application of magnetic field enhances the peak intensity of $\it{S_{xx}}$ at T $\sim$ 60 K. Additionally, $\it{S_{xx}(T)}$ curves measured at different fields exhibit a crossover at T = 20 K, which suggest the existence of unique feature in the CDW state of VSe$_2$ \textit{i.e.} a locally exact isosbestic point.
title Extended Kohler's scaling, a low temperature anomaly and Isosbestic point in the charge density wave state of 1T-VSe$_2$
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2405.15483