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Main Authors: Chiodini, Stefano, Venturi, Giacomo, Kerfoot, James, Zhang, Jincan, Alexeev, Evgeny M., Taniguchi, Takashi, Watanabe, Kenji, Ferrari, Andrea C., Ambrosio, Antonio
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2406.02195
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author Chiodini, Stefano
Venturi, Giacomo
Kerfoot, James
Zhang, Jincan
Alexeev, Evgeny M.
Taniguchi, Takashi
Watanabe, Kenji
Ferrari, Andrea C.
Ambrosio, Antonio
author_facet Chiodini, Stefano
Venturi, Giacomo
Kerfoot, James
Zhang, Jincan
Alexeev, Evgeny M.
Taniguchi, Takashi
Watanabe, Kenji
Ferrari, Andrea C.
Ambrosio, Antonio
contents In twisted layered materials (t-LMs), an inter-layer rotation can break inversion symmetry and create an interfacial array of staggered out-of-plane polarization due to AB/BA stacking registries. This symmetry breaking can also trigger the formation of edge in-plane polarizations localized along the perimeter of AB/BA regions (i.e., saddle point domains). However, a comprehensive experimental investigation of these features is still lacking. Here, we use piezo force microscopy to probe the electromechanical behavior of twisted hexagonal boron nitride (t-hBN). For a parallel stacking alignment of t-hBN, we reveal very narrow (width ~ 20 nm) saddle point polarizations, which we also measure in the anti-parallel configuration. These localized polarizations can still be found on a multiply-stacked t-hBN structure, determining the formation of a double moiré. We also visualize a t-hBN moiré superlattice in the topography maps with atomic force microscopy, related to the strain accumulated at the saddle point domains. Our findings imply that polarizations in t-hBN do not only point in the out-of-plane direction, but also show an in-plane component, giving rise to a much more complex 3D polarization field.
format Preprint
id arxiv_https___arxiv_org_abs_2406_02195
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Electromechanical response of saddle points in twisted hBN moiré superlattices
Chiodini, Stefano
Venturi, Giacomo
Kerfoot, James
Zhang, Jincan
Alexeev, Evgeny M.
Taniguchi, Takashi
Watanabe, Kenji
Ferrari, Andrea C.
Ambrosio, Antonio
Materials Science
In twisted layered materials (t-LMs), an inter-layer rotation can break inversion symmetry and create an interfacial array of staggered out-of-plane polarization due to AB/BA stacking registries. This symmetry breaking can also trigger the formation of edge in-plane polarizations localized along the perimeter of AB/BA regions (i.e., saddle point domains). However, a comprehensive experimental investigation of these features is still lacking. Here, we use piezo force microscopy to probe the electromechanical behavior of twisted hexagonal boron nitride (t-hBN). For a parallel stacking alignment of t-hBN, we reveal very narrow (width ~ 20 nm) saddle point polarizations, which we also measure in the anti-parallel configuration. These localized polarizations can still be found on a multiply-stacked t-hBN structure, determining the formation of a double moiré. We also visualize a t-hBN moiré superlattice in the topography maps with atomic force microscopy, related to the strain accumulated at the saddle point domains. Our findings imply that polarizations in t-hBN do not only point in the out-of-plane direction, but also show an in-plane component, giving rise to a much more complex 3D polarization field.
title Electromechanical response of saddle points in twisted hBN moiré superlattices
topic Materials Science
url https://arxiv.org/abs/2406.02195