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Main Authors: Chen, Tong, Siddiquee, Hasan, Rehfuss, Zack, Gao, Shiyuan, Lygouras, Chris, Drouin, Jack, Morano, Vincent, Avers, Keenan E., Schmitt, Christopher J., Podlesnyak, Andrey, Ran, Sheng, Song, Yu, Broholm, Collin
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2406.03566
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author Chen, Tong
Siddiquee, Hasan
Rehfuss, Zack
Gao, Shiyuan
Lygouras, Chris
Drouin, Jack
Morano, Vincent
Avers, Keenan E.
Schmitt, Christopher J.
Podlesnyak, Andrey
Ran, Sheng
Song, Yu
Broholm, Collin
author_facet Chen, Tong
Siddiquee, Hasan
Rehfuss, Zack
Gao, Shiyuan
Lygouras, Chris
Drouin, Jack
Morano, Vincent
Avers, Keenan E.
Schmitt, Christopher J.
Podlesnyak, Andrey
Ran, Sheng
Song, Yu
Broholm, Collin
contents The tetragonal heavy-fermion superconductor CeRh$_2$As$_2$ ($T_{\rm c}=0.3$ K) exhibits an exceptionally high critical field of 14 T for $\textbf{B} \parallel \textbf{c}$. It undergoes a field-driven first-order phase transition between superconducting (SC) states, potentially transitioning from spin-singlet to spin-triplet superconductivity. To elucidate the underlying pairing mechanism, we probe spin fluctuations in CeRh$_2$As$_2$ using neutron scattering. We find dynamic $(π,π)$ antiferromagnetic spin correlations with an anisotropic quasi-two-dimensional correlation volume. Our data place an upper limit of 0.31 $μ_{\rm B}$ on the staggered magnetization of corresponding Néel orders at $T=0.08$ K. Density functional theory (DFT) calculations, treating Ce $4f$ electrons as core states, show that the AFM wave vector connects significant areas of the Fermi surface. Our findings show the dominant excitations in CeRh$_2$As$_2$ for $\hbarω< 1.2$~meV are magnetic and indicate superconductivity in CeRh$_2$As$_2$ is mediated by AFM spin fluctuations associated with a proximate quantum critical point.
format Preprint
id arxiv_https___arxiv_org_abs_2406_03566
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Quasi-two-dimensional Antiferromagnetic Spin Fluctuations in the Spin-triplet Superconductor Candidate CeRh$_2$As$_2$
Chen, Tong
Siddiquee, Hasan
Rehfuss, Zack
Gao, Shiyuan
Lygouras, Chris
Drouin, Jack
Morano, Vincent
Avers, Keenan E.
Schmitt, Christopher J.
Podlesnyak, Andrey
Ran, Sheng
Song, Yu
Broholm, Collin
Strongly Correlated Electrons
Superconductivity
The tetragonal heavy-fermion superconductor CeRh$_2$As$_2$ ($T_{\rm c}=0.3$ K) exhibits an exceptionally high critical field of 14 T for $\textbf{B} \parallel \textbf{c}$. It undergoes a field-driven first-order phase transition between superconducting (SC) states, potentially transitioning from spin-singlet to spin-triplet superconductivity. To elucidate the underlying pairing mechanism, we probe spin fluctuations in CeRh$_2$As$_2$ using neutron scattering. We find dynamic $(π,π)$ antiferromagnetic spin correlations with an anisotropic quasi-two-dimensional correlation volume. Our data place an upper limit of 0.31 $μ_{\rm B}$ on the staggered magnetization of corresponding Néel orders at $T=0.08$ K. Density functional theory (DFT) calculations, treating Ce $4f$ electrons as core states, show that the AFM wave vector connects significant areas of the Fermi surface. Our findings show the dominant excitations in CeRh$_2$As$_2$ for $\hbarω< 1.2$~meV are magnetic and indicate superconductivity in CeRh$_2$As$_2$ is mediated by AFM spin fluctuations associated with a proximate quantum critical point.
title Quasi-two-dimensional Antiferromagnetic Spin Fluctuations in the Spin-triplet Superconductor Candidate CeRh$_2$As$_2$
topic Strongly Correlated Electrons
Superconductivity
url https://arxiv.org/abs/2406.03566