Stoichiometry-induced ferromagnetism in altermagnetic candidate MnTe
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arXiv
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| Natura: | Preprint |
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2024
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| author | Chilcote, Michael Mazza, Alessandro R. Lu, Qiangsheng Gray, Isaiah Tian, Qi Deng, Qinwen Moseley, Duncan Chen, An-Hsi Lapano, Jason Gardner, Jason S. Eres, Gyula Ward, T. Zac Feng, Erxi Cao, Huibo Lauter, Valeria McGuire, Michael A. Hermann, Raphael Parker, David Han, Myung-Geun Kayani, Asghar Rimal, Gaurab Wu, Liang Charlton, Timothy R. Moore, Robert G. Brahlek, Matthew |
| author_facet | Chilcote, Michael Mazza, Alessandro R. Lu, Qiangsheng Gray, Isaiah Tian, Qi Deng, Qinwen Moseley, Duncan Chen, An-Hsi Lapano, Jason Gardner, Jason S. Eres, Gyula Ward, T. Zac Feng, Erxi Cao, Huibo Lauter, Valeria McGuire, Michael A. Hermann, Raphael Parker, David Han, Myung-Geun Kayani, Asghar Rimal, Gaurab Wu, Liang Charlton, Timothy R. Moore, Robert G. Brahlek, Matthew |
| contents | The field of spintronics has seen a surge of interest in altermagnetism due to novel predictions and many possible applications. MnTe is a leading altermagnetic candidate that is of significant interest across spintronics due to its layered antiferromagnetic structure, high Neel temperature (TN ~ 310 K) and semiconducting properties. We present results on molecular beam epitaxy (MBE) grown MnTe/InP(111) films. Here, it is found that the electronic and magnetic properties are driven by the natural stoichiometry of MnTe. Electronic transport and in situ angle-resolved photoemission spectroscopy show the films are natively metallic with the Fermi level in the valence band and the band structure is in good agreement with first principles calculations for altermagnetic spin-splitting. Neutron diffraction confirms that the film is antiferromagnetic with planar anisotropy and polarized neutron reflectometry indicates weak ferromagnetism, which is linked to a slight Mn-richness that is intrinsic to the MBE grown samples. When combined with the anomalous Hall effect, this work shows that the electronic response is strongly affected by the ferromagnetic moment. Altogether, this highlights potential mechanisms for controlling altermagnetic ordering for diverse spintronic applications. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2406_04474 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | Stoichiometry-induced ferromagnetism in altermagnetic candidate MnTe Chilcote, Michael Mazza, Alessandro R. Lu, Qiangsheng Gray, Isaiah Tian, Qi Deng, Qinwen Moseley, Duncan Chen, An-Hsi Lapano, Jason Gardner, Jason S. Eres, Gyula Ward, T. Zac Feng, Erxi Cao, Huibo Lauter, Valeria McGuire, Michael A. Hermann, Raphael Parker, David Han, Myung-Geun Kayani, Asghar Rimal, Gaurab Wu, Liang Charlton, Timothy R. Moore, Robert G. Brahlek, Matthew Materials Science Other Condensed Matter The field of spintronics has seen a surge of interest in altermagnetism due to novel predictions and many possible applications. MnTe is a leading altermagnetic candidate that is of significant interest across spintronics due to its layered antiferromagnetic structure, high Neel temperature (TN ~ 310 K) and semiconducting properties. We present results on molecular beam epitaxy (MBE) grown MnTe/InP(111) films. Here, it is found that the electronic and magnetic properties are driven by the natural stoichiometry of MnTe. Electronic transport and in situ angle-resolved photoemission spectroscopy show the films are natively metallic with the Fermi level in the valence band and the band structure is in good agreement with first principles calculations for altermagnetic spin-splitting. Neutron diffraction confirms that the film is antiferromagnetic with planar anisotropy and polarized neutron reflectometry indicates weak ferromagnetism, which is linked to a slight Mn-richness that is intrinsic to the MBE grown samples. When combined with the anomalous Hall effect, this work shows that the electronic response is strongly affected by the ferromagnetic moment. Altogether, this highlights potential mechanisms for controlling altermagnetic ordering for diverse spintronic applications. |
| title | Stoichiometry-induced ferromagnetism in altermagnetic candidate MnTe |
| topic | Materials Science Other Condensed Matter |
| url | https://arxiv.org/abs/2406.04474 |