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Main Authors: Li, Zairui, Sims, Wesley, Shariatdoust, Mirali Seyed, Howell, Gabriel, Searles, Thomas A., Carbajo, Sergio
Format: Preprint
Published: 2024
Subjects:
Online Access:https://arxiv.org/abs/2406.04971
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_version_ 1866911910076612608
author Li, Zairui
Sims, Wesley
Shariatdoust, Mirali Seyed
Howell, Gabriel
Searles, Thomas A.
Carbajo, Sergio
author_facet Li, Zairui
Sims, Wesley
Shariatdoust, Mirali Seyed
Howell, Gabriel
Searles, Thomas A.
Carbajo, Sergio
contents Recent developments in high-power ultrafast optical technology and emerging theoretical frameworks in strong-field quantum electrodynamics (SF-QED) are unveiling nuanced differentiations between the semi-classical and full quantum mechanical descriptions of physical systems. Here we present a computational investigation of a novel technique for attosecond optical sensing through time correlation transduction (TCT) by investigating high-harmonic generation (HHG) as a representative SF-QED process. TCT is an experimental method to capture photon-electron interactions at higher harmonic orders by temporarily correlating the emitted and driving photon fields. This approach enables resolving the dynamical behavior of optically-driven strong-field phenomena in quantum materials such as Two-dimensional Materials and Dirac Semimetals down to 10 attosecond temporal resolution to discover a full quantum explanation. Predicting and measuring the transition between perturbative and non-perturbative regimes with attosecond resolution can deepen the understanding of SF-QED such as HHG. As such, we find that TCT is a powerful method to pave the way toward the functional characterization of quantum matter.
format Preprint
id arxiv_https___arxiv_org_abs_2406_04971
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Time-correlation Transduction in Strong-field Quantum Electrodynamics
Li, Zairui
Sims, Wesley
Shariatdoust, Mirali Seyed
Howell, Gabriel
Searles, Thomas A.
Carbajo, Sergio
Optics
81V10
F.1.2
Recent developments in high-power ultrafast optical technology and emerging theoretical frameworks in strong-field quantum electrodynamics (SF-QED) are unveiling nuanced differentiations between the semi-classical and full quantum mechanical descriptions of physical systems. Here we present a computational investigation of a novel technique for attosecond optical sensing through time correlation transduction (TCT) by investigating high-harmonic generation (HHG) as a representative SF-QED process. TCT is an experimental method to capture photon-electron interactions at higher harmonic orders by temporarily correlating the emitted and driving photon fields. This approach enables resolving the dynamical behavior of optically-driven strong-field phenomena in quantum materials such as Two-dimensional Materials and Dirac Semimetals down to 10 attosecond temporal resolution to discover a full quantum explanation. Predicting and measuring the transition between perturbative and non-perturbative regimes with attosecond resolution can deepen the understanding of SF-QED such as HHG. As such, we find that TCT is a powerful method to pave the way toward the functional characterization of quantum matter.
title Time-correlation Transduction in Strong-field Quantum Electrodynamics
topic Optics
81V10
F.1.2
url https://arxiv.org/abs/2406.04971