Phonon-induced renormalization of exchange interactions in metallic two-dimensional magnets

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Hauptverfasser: Badrtdinov, Danis I., Katsnelson, Mikhail I., Rudenko, Alexander N.
Format: Preprint
Veröffentlicht: 2024
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author Badrtdinov, Danis I.
Katsnelson, Mikhail I.
Rudenko, Alexander N.
author_facet Badrtdinov, Danis I.
Katsnelson, Mikhail I.
Rudenko, Alexander N.
contents The presence of spin-polarized charge carriers in metallic magnets provides a mechanism for spin-lattice interactions mediated by electron-phonon coupling. Here, we present a theory of this mechanism used to estimate its effect on the exchange interactions in 2D magnets. Starting from a square lattice model at half filling, we show that the presence of electron-phonon coupling with equilibrium phonon distribution leads to a notable suppression of exchange interactions with temperature. We then apply our approach to the prototypical 2D metallic ferromagnet, Fe$_3$GeTe$_2$, with moderate electron-phonon coupling. We find that the exchange interactions undergo a renormalization, leading to a softening of the magnon modes, and suppression of the Curie temperature by $\sim$10\%. We expect that this effect can be further enhanced in systems with strong electron-phonon coupling, as well as for non-equilibrium distribution of phonons induced by strong laser fields or charge currents.
format Preprint
id arxiv_https___arxiv_org_abs_2406_05229
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Phonon-induced renormalization of exchange interactions in metallic two-dimensional magnets
Badrtdinov, Danis I.
Katsnelson, Mikhail I.
Rudenko, Alexander N.
Materials Science
Strongly Correlated Electrons
The presence of spin-polarized charge carriers in metallic magnets provides a mechanism for spin-lattice interactions mediated by electron-phonon coupling. Here, we present a theory of this mechanism used to estimate its effect on the exchange interactions in 2D magnets. Starting from a square lattice model at half filling, we show that the presence of electron-phonon coupling with equilibrium phonon distribution leads to a notable suppression of exchange interactions with temperature. We then apply our approach to the prototypical 2D metallic ferromagnet, Fe$_3$GeTe$_2$, with moderate electron-phonon coupling. We find that the exchange interactions undergo a renormalization, leading to a softening of the magnon modes, and suppression of the Curie temperature by $\sim$10\%. We expect that this effect can be further enhanced in systems with strong electron-phonon coupling, as well as for non-equilibrium distribution of phonons induced by strong laser fields or charge currents.
title Phonon-induced renormalization of exchange interactions in metallic two-dimensional magnets
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2406.05229