Manipulating magnetism and transport properties of EuCd$_2$P$_2$ with a low carrier concentration

Fuente: arXiv
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Autori principali: Chen, Xiyu, Wang, Ziwen, Zhou, Zhiyu, Yang, Wuzhang, Liu, Yi, Lu, Jia-Yi, Ren, Zhi, Cao, Guang-Han, Tafti, Fazel, Dong, Shuai, Wang, Zhi-Cheng
Natura: Preprint
Pubblicazione: 2024
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author Chen, Xiyu
Wang, Ziwen
Zhou, Zhiyu
Yang, Wuzhang
Liu, Yi
Lu, Jia-Yi
Ren, Zhi
Cao, Guang-Han
Tafti, Fazel
Dong, Shuai
Wang, Zhi-Cheng
author_facet Chen, Xiyu
Wang, Ziwen
Zhou, Zhiyu
Yang, Wuzhang
Liu, Yi
Lu, Jia-Yi
Ren, Zhi
Cao, Guang-Han
Tafti, Fazel
Dong, Shuai
Wang, Zhi-Cheng
contents Materials that exhibit strongly coupled magnetic order and electronic properties are crucial for both fundamental research and technological applications. However, finding a material that not only shows remarkable magnetoresistive responses but also has an easily tunable ground state remains a challenge. Here, we report successful manipulation of the magnetic and transport properties of EuCd$_2$P$_2$, which is transformed from an A-type antiferromagnet ($T_\mathrm{N}$ = 11 K) exhibiting colossal magnetoresistance into a ferromagnet ($T_\mathrm{C}$ = 47 K) with metallic behavior. The dramatic alteration results from a low hole concentration of $10^{19}$ cm$^{-3}$ induced by changing the growth conditions. Electronic structure and total energy calculations confirm the tunability of magnetism with a small carrier concentration for EuCd$_2$P$_2$. It is feasible to switch between the magnetic states by using field-effect to control the carrier density, thereby changing the magneto-electronic response. The controllable magnetism and electrical transport of EuCd$_2$P$_2$ make it a potential candidate for spintronics.
format Preprint
id arxiv_https___arxiv_org_abs_2406_05823
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Manipulating magnetism and transport properties of EuCd$_2$P$_2$ with a low carrier concentration
Chen, Xiyu
Wang, Ziwen
Zhou, Zhiyu
Yang, Wuzhang
Liu, Yi
Lu, Jia-Yi
Ren, Zhi
Cao, Guang-Han
Tafti, Fazel
Dong, Shuai
Wang, Zhi-Cheng
Materials Science
Strongly Correlated Electrons
Materials that exhibit strongly coupled magnetic order and electronic properties are crucial for both fundamental research and technological applications. However, finding a material that not only shows remarkable magnetoresistive responses but also has an easily tunable ground state remains a challenge. Here, we report successful manipulation of the magnetic and transport properties of EuCd$_2$P$_2$, which is transformed from an A-type antiferromagnet ($T_\mathrm{N}$ = 11 K) exhibiting colossal magnetoresistance into a ferromagnet ($T_\mathrm{C}$ = 47 K) with metallic behavior. The dramatic alteration results from a low hole concentration of $10^{19}$ cm$^{-3}$ induced by changing the growth conditions. Electronic structure and total energy calculations confirm the tunability of magnetism with a small carrier concentration for EuCd$_2$P$_2$. It is feasible to switch between the magnetic states by using field-effect to control the carrier density, thereby changing the magneto-electronic response. The controllable magnetism and electrical transport of EuCd$_2$P$_2$ make it a potential candidate for spintronics.
title Manipulating magnetism and transport properties of EuCd$_2$P$_2$ with a low carrier concentration
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2406.05823