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Autori principali: Zhao, Weiyao, Trang, Chi Xuan, Li, Qile, Chen, Lei, Yue, Zengji, Bake, Abdulhakim, Tan, Cheng, Wang, Lan, Nancarrow, Mitchell, Edmonds, Mark, Cortie, David, Wang, Xiaolin
Natura: Preprint
Pubblicazione: 2024
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Accesso online:https://arxiv.org/abs/2406.09628
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author Zhao, Weiyao
Trang, Chi Xuan
Li, Qile
Chen, Lei
Yue, Zengji
Bake, Abdulhakim
Tan, Cheng
Wang, Lan
Nancarrow, Mitchell
Edmonds, Mark
Cortie, David
Wang, Xiaolin
author_facet Zhao, Weiyao
Trang, Chi Xuan
Li, Qile
Chen, Lei
Yue, Zengji
Bake, Abdulhakim
Tan, Cheng
Wang, Lan
Nancarrow, Mitchell
Edmonds, Mark
Cortie, David
Wang, Xiaolin
contents Topological insulators (TIs) are emergent materials with unique band structure, which allow the study of quantum effect in solids, as well as contribute to high performance quantum devices. To achieve the better performance of TI, here we present a co-doping strategy using synergistic rare-earth Sm and transition-metal Fe dopants in Bi2Se3 single crystals, which combine the advantages of both transition metal doped TI (high ferromagnetic ordering temperature and observed QAHE), and rare-earth doped TI (large magnetic moments and significant spin orbit coupling). In the as-grown single crystals, clear evidences of ferromagnetic ordering were observed. The angle resolve photoemission spectroscopy indicate the ferromagnetism opens a 44 meV band gap at surface Dirac point. Moreover, the carrier mobility at 3 K is ~ 7400 cm2/Vs, and we thus observed an ultra-strong Shubnikov-de Haas oscillation in the longitudinal resistivity, as well as the Hall steps in transverse resistivity below 14 T. Our transport and angular resolved photoemission spectroscopy results suggest that the rare-earth and transition metal co-doping in Bi2Se3 system is a promising avenue implement the quantum anomalous Hall effect, as well as harnessing the massive Dirac fermion in electrical devices.
format Preprint
id arxiv_https___arxiv_org_abs_2406_09628
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Massive Dirac Fermions and Strong Shubnikov-de Haas Oscillations in Topological Insulator Sm,Fe:Bi2Se3 Single Crystals
Zhao, Weiyao
Trang, Chi Xuan
Li, Qile
Chen, Lei
Yue, Zengji
Bake, Abdulhakim
Tan, Cheng
Wang, Lan
Nancarrow, Mitchell
Edmonds, Mark
Cortie, David
Wang, Xiaolin
Materials Science
Topological insulators (TIs) are emergent materials with unique band structure, which allow the study of quantum effect in solids, as well as contribute to high performance quantum devices. To achieve the better performance of TI, here we present a co-doping strategy using synergistic rare-earth Sm and transition-metal Fe dopants in Bi2Se3 single crystals, which combine the advantages of both transition metal doped TI (high ferromagnetic ordering temperature and observed QAHE), and rare-earth doped TI (large magnetic moments and significant spin orbit coupling). In the as-grown single crystals, clear evidences of ferromagnetic ordering were observed. The angle resolve photoemission spectroscopy indicate the ferromagnetism opens a 44 meV band gap at surface Dirac point. Moreover, the carrier mobility at 3 K is ~ 7400 cm2/Vs, and we thus observed an ultra-strong Shubnikov-de Haas oscillation in the longitudinal resistivity, as well as the Hall steps in transverse resistivity below 14 T. Our transport and angular resolved photoemission spectroscopy results suggest that the rare-earth and transition metal co-doping in Bi2Se3 system is a promising avenue implement the quantum anomalous Hall effect, as well as harnessing the massive Dirac fermion in electrical devices.
title Massive Dirac Fermions and Strong Shubnikov-de Haas Oscillations in Topological Insulator Sm,Fe:Bi2Se3 Single Crystals
topic Materials Science
url https://arxiv.org/abs/2406.09628