Chiral excitonic systems in twisted bilayers from Förster coupling and unconventional excitonic Hall effects

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Hauptverfasser: Li, Ci, Yao, Wang
Format: Preprint
Veröffentlicht: 2024
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author Li, Ci
Yao, Wang
author_facet Li, Ci
Yao, Wang
contents In twisted bilayer semiconductors with arbitrary twisting angles, a chiral excitonic system can arise from the interlayer electron-hole Coulomb exchange interaction (Förster coupling) that hybridizes the anisotropic intralayer excitons from individual layers. We present a general framework for the effective exciton Hamiltonian taking into account the electron-hole Coulomb exchange, using twisted homobilayer systems composed of transition metal dichalcogenides or black phosphorus as examples. We demonstrate that such chiral excitonic systems can feature unconventional Hall (Nernst) effects arising from quantum geometric properties characteristic of the layer hybridized wavefunctions under the chiral symmetry, for example, the time-reversal even layer Hall counter flow and the crossed nonlinear dynamical Hall effect, when mechanical and statistical force (temperature or density gradient) drives the exciton flow.
format Preprint
id arxiv_https___arxiv_org_abs_2406_09674
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Chiral excitonic systems in twisted bilayers from Förster coupling and unconventional excitonic Hall effects
Li, Ci
Yao, Wang
Mesoscale and Nanoscale Physics
In twisted bilayer semiconductors with arbitrary twisting angles, a chiral excitonic system can arise from the interlayer electron-hole Coulomb exchange interaction (Förster coupling) that hybridizes the anisotropic intralayer excitons from individual layers. We present a general framework for the effective exciton Hamiltonian taking into account the electron-hole Coulomb exchange, using twisted homobilayer systems composed of transition metal dichalcogenides or black phosphorus as examples. We demonstrate that such chiral excitonic systems can feature unconventional Hall (Nernst) effects arising from quantum geometric properties characteristic of the layer hybridized wavefunctions under the chiral symmetry, for example, the time-reversal even layer Hall counter flow and the crossed nonlinear dynamical Hall effect, when mechanical and statistical force (temperature or density gradient) drives the exciton flow.
title Chiral excitonic systems in twisted bilayers from Förster coupling and unconventional excitonic Hall effects
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2406.09674