Efficient production of $^{229m}$Th via nuclear excitation by electron capture

Fuente: arXiv
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Main Authors: Zhao, Jingyan, Pálffy, Adriana, Keitel, Christoph H., Wu, Yuanbin
Format: Preprint
Published: 2024
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author Zhao, Jingyan
Pálffy, Adriana
Keitel, Christoph H.
Wu, Yuanbin
author_facet Zhao, Jingyan
Pálffy, Adriana
Keitel, Christoph H.
Wu, Yuanbin
contents The nuclear isomeric state $^{229m}$Th with an exceptionally low excitation energy makes the $^{229}$Th isotope a crucial candidate for nuclear clocks and many other applications. Efficient and controllable production of $^{229m}$Th is essential and still remains a challenge. Here we report a novel approach for efficient production of $^{229m}$Th by the excitation of $^{229}$Th to the above-lying excited state at $29.19$ keV energy via the process of nuclear excitation by electron capture (NEEC). We show theoretically that the production rate of $^{229m}$Th per nucleus with accessible conditions can be six orders of magnitude larger than the value experimentally demonstrated using $29$-keV synchrotron radiation for this indirect excitation. With the efficient production of $^{229m}$Th, our results identify scenarios, as well as the characteristic NEEC signature with which NEEC events could be unambiguously identified, for a clear experimental identification of the long-sought NEEC phenomenon.
format Preprint
id arxiv_https___arxiv_org_abs_2406_12497
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Efficient production of $^{229m}$Th via nuclear excitation by electron capture
Zhao, Jingyan
Pálffy, Adriana
Keitel, Christoph H.
Wu, Yuanbin
Nuclear Theory
The nuclear isomeric state $^{229m}$Th with an exceptionally low excitation energy makes the $^{229}$Th isotope a crucial candidate for nuclear clocks and many other applications. Efficient and controllable production of $^{229m}$Th is essential and still remains a challenge. Here we report a novel approach for efficient production of $^{229m}$Th by the excitation of $^{229}$Th to the above-lying excited state at $29.19$ keV energy via the process of nuclear excitation by electron capture (NEEC). We show theoretically that the production rate of $^{229m}$Th per nucleus with accessible conditions can be six orders of magnitude larger than the value experimentally demonstrated using $29$-keV synchrotron radiation for this indirect excitation. With the efficient production of $^{229m}$Th, our results identify scenarios, as well as the characteristic NEEC signature with which NEEC events could be unambiguously identified, for a clear experimental identification of the long-sought NEEC phenomenon.
title Efficient production of $^{229m}$Th via nuclear excitation by electron capture
topic Nuclear Theory
url https://arxiv.org/abs/2406.12497