Design and Performance of a Magnetic Bottle Electron Spectrometer for High-Energy Photoelectron Spectroscopy

Fuente: arXiv
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Hauptverfasser: Borne, Kurtis, ONeal, Jordan T, Wang, Jun, Isele, Erk, Obaid, Razib, Berrah, Nora, Cheng, Xinxin, Bucksbaum, Philip H, James, Justin, Kamalov, Andri, Larsen, Kirk A, Li, Xiang, Lin, Ming-Fu, Liu, Yusong, Marinelli, Agostino, Summers, Adam, Thierstein, Emily, Wolf, Thomas, Rolles, Daniel, Walter, Peter, Cryan, James P, Driver, Taran
Format: Preprint
Veröffentlicht: 2024
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author Borne, Kurtis
ONeal, Jordan T
Wang, Jun
Isele, Erk
Obaid, Razib
Berrah, Nora
Cheng, Xinxin
Bucksbaum, Philip H
James, Justin
Kamalov, Andri
Larsen, Kirk A
Li, Xiang
Lin, Ming-Fu
Liu, Yusong
Marinelli, Agostino
Summers, Adam
Thierstein, Emily
Wolf, Thomas
Rolles, Daniel
Walter, Peter
Cryan, James P
Driver, Taran
author_facet Borne, Kurtis
ONeal, Jordan T
Wang, Jun
Isele, Erk
Obaid, Razib
Berrah, Nora
Cheng, Xinxin
Bucksbaum, Philip H
James, Justin
Kamalov, Andri
Larsen, Kirk A
Li, Xiang
Lin, Ming-Fu
Liu, Yusong
Marinelli, Agostino
Summers, Adam
Thierstein, Emily
Wolf, Thomas
Rolles, Daniel
Walter, Peter
Cryan, James P
Driver, Taran
contents We describe the design and performance of a magnetic bottle electron spectrometer~(MBES) for high-energy electron spectroscopy. Our design features a ${\sim2}$~m long electron drift tube and electrostatic retardation lens, achieving sub-electronvolt (eV) electron kinetic energy resolution for high energy (several hundred eV) electrons with close to 4$π$ collection efficiency. A segmented anode electron detector enables the simultaneous collection of photoelectron spectra in high resolution and high collection efficiency modes. This versatile instrument is installed at the TMO endstation at the LCLS x-ray free-electron laser (XFEL). In this paper, we demonstrate its high resolution, collection efficiency and spatial selectivity in measurements where it is coupled to an XFEL source. These combined characteristics are designed to enable high-resolution time-resolved measurements using x-ray photoelectron, absorption, and Auger-Meitner spectroscopy. We also describe the pervasive artifact in MBES time-of-flight spectra that arises from a periodic modulation in electron detection efficiency, and present a robust analysis procedure for its removal.
format Preprint
id arxiv_https___arxiv_org_abs_2406_13083
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Design and Performance of a Magnetic Bottle Electron Spectrometer for High-Energy Photoelectron Spectroscopy
Borne, Kurtis
ONeal, Jordan T
Wang, Jun
Isele, Erk
Obaid, Razib
Berrah, Nora
Cheng, Xinxin
Bucksbaum, Philip H
James, Justin
Kamalov, Andri
Larsen, Kirk A
Li, Xiang
Lin, Ming-Fu
Liu, Yusong
Marinelli, Agostino
Summers, Adam
Thierstein, Emily
Wolf, Thomas
Rolles, Daniel
Walter, Peter
Cryan, James P
Driver, Taran
Instrumentation and Detectors
We describe the design and performance of a magnetic bottle electron spectrometer~(MBES) for high-energy electron spectroscopy. Our design features a ${\sim2}$~m long electron drift tube and electrostatic retardation lens, achieving sub-electronvolt (eV) electron kinetic energy resolution for high energy (several hundred eV) electrons with close to 4$π$ collection efficiency. A segmented anode electron detector enables the simultaneous collection of photoelectron spectra in high resolution and high collection efficiency modes. This versatile instrument is installed at the TMO endstation at the LCLS x-ray free-electron laser (XFEL). In this paper, we demonstrate its high resolution, collection efficiency and spatial selectivity in measurements where it is coupled to an XFEL source. These combined characteristics are designed to enable high-resolution time-resolved measurements using x-ray photoelectron, absorption, and Auger-Meitner spectroscopy. We also describe the pervasive artifact in MBES time-of-flight spectra that arises from a periodic modulation in electron detection efficiency, and present a robust analysis procedure for its removal.
title Design and Performance of a Magnetic Bottle Electron Spectrometer for High-Energy Photoelectron Spectroscopy
topic Instrumentation and Detectors
url https://arxiv.org/abs/2406.13083