Spectroscopy of Hubbard-Mott excitons and their ro-vibrational excitations

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Hauptverfasser: Bohrdt, Annabelle, Demler, Eugene, Grusdt, Fabian
Format: Preprint
Veröffentlicht: 2024
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author Bohrdt, Annabelle
Demler, Eugene
Grusdt, Fabian
author_facet Bohrdt, Annabelle
Demler, Eugene
Grusdt, Fabian
contents Hubbard excitons are bound states of doublons and holes that can be experimentally probed both in real materials, such as cuprates, and in cold atom quantum simulators. Here we compare properties of a Hubbard exciton to those of a pair of distinguishable dopants in the $t-J$ model and show how insights into pair properties can be obtained through excitonic spectra. In particular, we perform large-scale numerical simulations of spectral functions and optical conductivities and obtain remarkable agreement between Hubbard excitons and pairs of distinguishable dopants. The latter can be decomposed into symmetric (bosonic) and anti-symmetric (fermionic) sectors of indistinguishable dopants, thus enabling a detailed understanding of different features observed in the excitonic spectra through comparison with a semi-analytical geometric string theory approach. We further compare theoretically computed exciton spectra in a single band Fermi-Hubbard model to resonant inelastic X-ray scattering (RIXS) studies of the parent insulating cuprate materials. We find remarkable agreement between the two spectra in both energy and momentum dependence. Our analysis suggests that multiple long-lived ro-vibrational exciton resonances have been observed in RIXS spectra. Experimentally, these features are known to persist up to optimal doping. The comparison we provide between semi-analytical theory, large-scale numerics, and experimental data thus provides an explanation of the RIXS measurements and provides new insight into the nature of pairing in cuprates.
format Preprint
id arxiv_https___arxiv_org_abs_2406_16854
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Spectroscopy of Hubbard-Mott excitons and their ro-vibrational excitations
Bohrdt, Annabelle
Demler, Eugene
Grusdt, Fabian
Strongly Correlated Electrons
Quantum Gases
Hubbard excitons are bound states of doublons and holes that can be experimentally probed both in real materials, such as cuprates, and in cold atom quantum simulators. Here we compare properties of a Hubbard exciton to those of a pair of distinguishable dopants in the $t-J$ model and show how insights into pair properties can be obtained through excitonic spectra. In particular, we perform large-scale numerical simulations of spectral functions and optical conductivities and obtain remarkable agreement between Hubbard excitons and pairs of distinguishable dopants. The latter can be decomposed into symmetric (bosonic) and anti-symmetric (fermionic) sectors of indistinguishable dopants, thus enabling a detailed understanding of different features observed in the excitonic spectra through comparison with a semi-analytical geometric string theory approach. We further compare theoretically computed exciton spectra in a single band Fermi-Hubbard model to resonant inelastic X-ray scattering (RIXS) studies of the parent insulating cuprate materials. We find remarkable agreement between the two spectra in both energy and momentum dependence. Our analysis suggests that multiple long-lived ro-vibrational exciton resonances have been observed in RIXS spectra. Experimentally, these features are known to persist up to optimal doping. The comparison we provide between semi-analytical theory, large-scale numerics, and experimental data thus provides an explanation of the RIXS measurements and provides new insight into the nature of pairing in cuprates.
title Spectroscopy of Hubbard-Mott excitons and their ro-vibrational excitations
topic Strongly Correlated Electrons
Quantum Gases
url https://arxiv.org/abs/2406.16854